Well-defined assembly of plasmonic metal nanoparticles by dielectrophoresis for highly sensitive SERS-active substrates
In this study, dielectrophoresis (DEP) was performed to develop highly sensitive surface- enhanced Raman scattering (SERS)-active substrates for molecular sensing. Substrates with a circular hole pattern were used, and plasmonic particles were trapped and immobilized along the edges of the pattern using dielectrophoretic forces. The arranged particles created hotspots, resulting in an enhanced SERS signal that was detectable even at concentrations as low as 10<sup>-10</sup> M. This uniform arrangement provided a consistent signal over a large area. In addition, it was experimentally verified that the behavior of the particles varied with pattern diameter. This phenomenon was further supported by theoretical analysis. The proposed DEP-based SERS substrates are expected to be useful in various applications due to their excellent reproducibility and reliability.
Authors
- Gyu Leem (ORCID: https://orcid.org/0000-0003-0169-1096)
- Sunghoon Yoo (ORCID: https://orcid.org/0000-0002-1568-9651)
- Tae Jae Lee
- Dong Hwan Nam (ORCID: https://orcid.org/0000-0002-8641-4540)
- Jae‐Sung Kwon (ORCID: https://orcid.org/0000-0002-7854-2964)
- Seunghyun Lee (ORCID: https://orcid.org/0000-0002-2477-1243)
- Ha Young Kim (ORCID: https://orcid.org/0000-0001-5115-9984)
- Jae‐Jun Park (ORCID: https://orcid.org/0000-0003-4643-1984)
- Y.C. Yeo
Institutions
- State University of New York (US)
- Incheon National University (KR)
- SUNY College of Environmental Science and Forestry (US)
- York University (US)
- National NanoFab Center (KR)
- Hanyang University (KR)
- Anyang University (KR)
Publication Details
- Journal
- Lab on a Chip
- Published
- 2025-01-01
- DOI
- https://doi.org/10.1039/d5lc00238a
- Citations
- 1
- Primary Topic
- Gold and Silver Nanoparticles Synthesis and Applications
- Type
- article
- Field-Weighted Citation Impact
- 0.43
Funders
- National Research Foundation
- Ministry of Trade, Industry and Energy
- National Research Foundation of Korea
- Gyeonggi-do Regional Research Center
- Ministry of Science and ICT, South Korea