Pseudogap and Fermi arc induced by Fermi surface nesting in a centrosymmetric skyrmion magnet

Skyrmions in noncentrosymmetric materials are believed to occur due to the Dzyaloshinskii-Moriya interaction. By contrast, the skyrmion formation mechanism in centrosymmetric materials remains elusive. Here, we reveal the intrinsic electronic structure of the centrosymmetric GdRu<sub>2</sub>Si<sub>2</sub> by selectively measuring magnetic domains using angle-resolved photoemission spectroscopy (ARPES). We found robust Fermi surface (FS) nesting, consistent with the magnetic modulation <b><i>q</i></b>-vector detected by the previous resonant x-ray scattering measurements. The pseudogap opens at the nested FS portions, which vary for different magnetic domains. The anomalous pseudogap disconnects the FS to generate Fermi arcs with twofold symmetry. These results indicate that the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction plays a decisive role in generating the screw spin modulation responsible for the skyrmion formation in GdRu<sub>2</sub>Si<sub>2</sub>. Furthermore, we demonstrate the flexible nature of magnetism in GdRu<sub>2</sub>Si<sub>2</sub> by manipulating magnetic domains with magnetic field and temperature cyclings, providing potential future applications for data storage and processing devices.

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Publication Details

Journal
Science
Published
2025-05-08
DOI
https://doi.org/10.1126/science.adj7710
Citations
8
Primary Topic
Magnetic properties of thin films
Type
article
Field-Weighted Citation Impact
9.97
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article

Pseudogap and Fermi arc induced by Fermi surface nesting in a centrosymmetric skyrmion magnet

Soonsang Huh, Tatsuma D. Matsuda, Yuji Aoki, Ryuji Higashinaka et al.
8 citations
Science
Magnetic properties of thin films
9.97
article

Pseudogap and Fermi arc induced by Fermi surface nesting in a centrosymmetric skyrmion magnet

Soonsang Huh, Tatsuma D. Matsuda, Yuji Aoki, Ryuji Higashinaka, Yuxuan Wan, Masayuki Ochi, Takeshi Kondo, Dong-Hui Lu, Masashi Tokunaga, Satoru Hayami, Yuyang Dong, Yuto Kinoshita, Makoto Hashimoto, Ryu Nakachi, Yosuke Arai
article en
8 citations

Abstract

Skyrmions in noncentrosymmetric materials are believed to occur due to the Dzyaloshinskii-Moriya interaction. By contrast, the skyrmion formation mechanism in centrosymmetric materials remains elusive. Here, we reveal the intrinsic electronic structure of the centrosymmetric GdRu<sub>2</sub>Si<sub>2</sub> by selectively measuring magnetic domains using angle-resolved photoemission spectroscopy (ARPES). We found robust Fermi surface (FS) nesting, consistent with the magnetic modulation <b><i>q</i></b>-vector detected by the previous resonant x-ray scattering measurements. The pseudogap opens at the nested FS portions, which vary for different magnetic domains. The anomalous pseudogap disconnects the FS to generate Fermi arcs with twofold symmetry. These results indicate that the Ruderman-Kittel-Kasuya-Yosida (RKKY) interaction plays a decisive role in generating the screw spin modulation responsible for the skyrmion formation in GdRu<sub>2</sub>Si<sub>2</sub>. Furthermore, we demonstrate the flexible nature of magnetism in GdRu<sub>2</sub>Si<sub>2</sub> by manipulating magnetic domains with magnetic field and temperature cyclings, providing potential future applications for data storage and processing devices.

ScienceVol. 388(6747)
Hokkaido University (JP), SLAC National Accelerator Laboratory (US), Stanford Synchrotron Radiation Lightsource (US), Tokyo Metropolitan University (JP), The University of Tokyo (JP), The University of Osaka (JP)
Openalex Percentile: Top 2%
Magnetic properties of thin films
9.97
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