Sustainable sodium alginate hydrogels incorporating banana leaf activated carbon and organo-clay for enhanced dye removal
New sodium alginate-based hydrogels using activated carbon from banana leaves and organo-modified montmorillonite for water treatment. Activated carbon extracted successfully from banana leaves and montmorillonite clay was surface-modified using cetyltrimethylammonium bromide as a cationic surfactant. Hydrogels were then synthesized using calcium chloride as the cross-linking agent. They were characterized using FTIR, X-ray diffraction, and scanning electronic microscopy. Characterization intimated the incorporation of components successfully. Adsorption performance was determined using pH, adsorbent dosages, initial dye concentration, and contact time. Sodium alginate-based hydrogels demonstrated remarkable efficacy in removing MB and EBT dyes from synthetic solutions, achieving removal efficiencies of up to 80.3% and 84.9% respectively within 90 min at pH 7. The adsorption process corresponded better to the Freundlich isotherm model. The kinetics of EBT dye removal were described by a pseudo-second-order model. Meanwhile, the kinetics of the removal of MB dyes were described by both pseudo-first order and intraparticle diffusion models. We conducted MTT assays to determine the cytotoxicity of our blends. This showed a dose-dependent drop in viability. Sodium alginate-based hydrogels made the cells least cytotoxic. The developed hydrogels can be used as safe and effective agents for water treatment, as indicated by the results.
Authors
- Ali H. M. Osman
- Zienab E. Eldin
- Mohamed Izham Mohamed Ibrahim (ORCID: https://orcid.org/0000-0001-9757-3574)
- Esraa G. Arafa
- Omayma Fawzy Abdel Gawad
- Shimaa Ahmed Abd-Elghafour
Institutions
- Beni-Suef University (EG)
- King Salman International University
Publication Details
- Journal
- Scientific Reports
- Published
- 2025-05-09
- DOI
- https://doi.org/10.1038/s41598-025-99343-8
- Citations
- 11
- Primary Topic
- Adsorption and biosorption for pollutant removal
- Type
- article
- Field-Weighted Citation Impact
- 8.99
Funders
- Beni-Suef University
- Science and Technology Development Fund