Subangstrom ion beam engineering of buried ultrathin oxides for scalable quantum computing
Multilayer nanoscale systems incorporating ultrathin tunnel barriers, magnetic materials, amorphous oxides, and promising dielectrics are essential for next-generation logics, memory, quantum, and neuro-inspired computing. Still, an ultrathin film control at the atomic scale remains challenging. Here, we introduce a complementary metal-oxide semiconductor-compatible approach using focused ion beam irradiation for buried ultrathin films' engineering with subangstrom thickness control. Molecular dynamics simulations confirm the pivotal role of ion-induced crystal defects. Its performance is exemplified by Josephson junction resistance tuning in the range of 2 to 37% with a 0.86% standard deviation in completed chips. Furthermore, it enables ±17-megahertz frequency accuracy (±0.172 angstrom tunnel barrier thickness variation) in superconducting multiqubit processors, as well as qubit energy relaxation and echo coherence times exceeding 0.5 milliseconds.
Authors
- Ilya A. Ryzhikov
- Vladimir V. Echeistov (ORCID: https://orcid.org/0000-0002-2258-9843)
- Nikita D. Korshakov (ORCID: https://orcid.org/0009-0008-5768-231X)
- A. V. Yanilkin (ORCID: https://orcid.org/0000-0002-7457-9911)
- E. V. Zikiy (ORCID: https://orcid.org/0000-0003-0473-7563)
- Elizaveta A. Krivko (ORCID: https://orcid.org/0009-0005-9952-4000)
- Elizaveta I. Malevannaya (ORCID: https://orcid.org/0000-0002-3298-8856)
- Viktor I. Polozov
- Dmitry O. Moskalev (ORCID: https://orcid.org/0000-0001-8446-6059)
- Ilya A. Rodionov (ORCID: https://orcid.org/0000-0002-8931-5142)
- Nikita S. Smirnov (ORCID: https://orcid.org/0000-0003-4097-5761)
- Aleksei R. Matanin (ORCID: https://orcid.org/0000-0003-4746-8455)
- A. V. Lebedev (ORCID: https://orcid.org/0000-0003-3653-8526)
- Аnton I. Ivanov (ORCID: https://orcid.org/0000-0002-7208-259X)
- Igor S. Korobenko
- Daria A. Moskaleva (ORCID: https://orcid.org/0000-0002-4649-5841)
- M. Teleganov
- Nikolai M. Zhitkov
- Ruslan V. Romashkin
- Aleksander V. Andriyash
- Anna Solovieva
- Dmitry A. Mikhalin (ORCID: https://orcid.org/0009-0004-9944-8135)
Institutions
- Bauman Moscow State Technical University (RU)
- All Russia Research Institute of Automatics (RU)
- Institute of Theoretical and Applied Electrodynamics (RU)
Publication Details
- Journal
- Science Advances
- Published
- 2025-05-07
- DOI
- https://doi.org/10.1126/sciadv.ads9744
- Citations
- 2
- Primary Topic
- Semiconductor materials and devices
- Type
- article
- Field-Weighted Citation Impact
- 1.46