Epitaxial Growth of AlGaN/AlN Strained-Layer Superlattices by Metalorganic Vapor Phase Epitaxy for Far-UV Second Harmonic Generation

Ultrathin AlN (<100 nm) layers fabricated via sputtering and subsequent face-to-face annealing (SP-FFA) over sapphire substrates can be applied as templates for the growth of AlGaN/AlN-based second harmonic generation (SHG) devices due to the high crystalline quality and smooth surface. This paper provides a concise overview of the crystalline characteristics of SP-FFA and metalorganic vapor phase epitaxy. An atomic force microscopy obtained a root-mean-square (RMS) roughness of 0.13 nm after the ultrathin growth of SP-FFA AlN. Subsequently, the impact of the SP-FFA AlN template on the regrowth of AlN and AlGaN by metalorganic vapor phase epitaxy has been examined. The phenomenon of the strong composition-pulling effect for the growth of AlGaN on the SP-FFA AlN template has been discussed. Finally, the paper discusses the successful growth of Al0.88Ga0.12N/AlN strained-layer superlattices, while ensuring a smooth surface morphology with an RMS roughness value of 0.15 nm, which effectively reduces the scattering loss in a waveguide. The growth of the strained-layer superlattice augments the nonlinear coupling coefficient kappa by utilizing the piezoelectric field in the transverse quasi-phase matching SHG device.

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Publication Details

Journal
Crystal Growth & Design
Published
2025-05-07
DOI
https://doi.org/10.1021/acs.cgd.4c01325
Citations
2
Primary Topic
GaN-based semiconductor devices and materials
Type
article
Field-Weighted Citation Impact
2.52

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article

Epitaxial Growth of AlGaN/AlN Strained-Layer Superlattices by Metalorganic Vapor Phase Epitaxy for Far-UV Second Harmonic Generation

Tomoyuki Tanikawa, Ryuji Katayama, Masahiro Uemukai, Hideto Miyake et al.
2 citations
Crystal Growth & Design
GaN-based semiconductor devices and materials
2.52
article

Epitaxial Growth of AlGaN/AlN Strained-Layer Superlattices by Metalorganic Vapor Phase Epitaxy for Far-UV Second Harmonic Generation

Tomoyuki Tanikawa, Ryuji Katayama, Masahiro Uemukai, Hideto Miyake, Hiroto Honda, Ryosuke Noro, Kanako Shojiki, Shahzeb Malik, Masaaki Ito
article en
2 citations

Abstract

Ultrathin AlN (<100 nm) layers fabricated via sputtering and subsequent face-to-face annealing (SP-FFA) over sapphire substrates can be applied as templates for the growth of AlGaN/AlN-based second harmonic generation (SHG) devices due to the high crystalline quality and smooth surface. This paper provides a concise overview of the crystalline characteristics of SP-FFA and metalorganic vapor phase epitaxy. An atomic force microscopy obtained a root-mean-square (RMS) roughness of 0.13 nm after the ultrathin growth of SP-FFA AlN. Subsequently, the impact of the SP-FFA AlN template on the regrowth of AlN and AlGaN by metalorganic vapor phase epitaxy has been examined. The phenomenon of the strong composition-pulling effect for the growth of AlGaN on the SP-FFA AlN template has been discussed. Finally, the paper discusses the successful growth of Al0.88Ga0.12N/AlN strained-layer superlattices, while ensuring a smooth surface morphology with an RMS roughness value of 0.15 nm, which effectively reduces the scattering loss in a waveguide. The growth of the strained-layer superlattice augments the nonlinear coupling coefficient kappa by utilizing the piezoelectric field in the transverse quasi-phase matching SHG device.

Crystal Growth & DesignVol. 25(10)
Mie University (JP), Kyoto University (JP), Quantum (Australia) (AU), Spintronics Research Network of Japan (JP), Graduate School USA (US)
Japan Society for the Promotion of Science
Openalex Percentile: Top 12%
GaN-based semiconductor devices and materials
2.52
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