Epitaxial Growth of AlGaN/AlN Strained-Layer Superlattices by Metalorganic Vapor Phase Epitaxy for Far-UV Second Harmonic Generation
Ultrathin AlN (<100 nm) layers fabricated via sputtering and subsequent face-to-face annealing (SP-FFA) over sapphire substrates can be applied as templates for the growth of AlGaN/AlN-based second harmonic generation (SHG) devices due to the high crystalline quality and smooth surface. This paper provides a concise overview of the crystalline characteristics of SP-FFA and metalorganic vapor phase epitaxy. An atomic force microscopy obtained a root-mean-square (RMS) roughness of 0.13 nm after the ultrathin growth of SP-FFA AlN. Subsequently, the impact of the SP-FFA AlN template on the regrowth of AlN and AlGaN by metalorganic vapor phase epitaxy has been examined. The phenomenon of the strong composition-pulling effect for the growth of AlGaN on the SP-FFA AlN template has been discussed. Finally, the paper discusses the successful growth of Al0.88Ga0.12N/AlN strained-layer superlattices, while ensuring a smooth surface morphology with an RMS roughness value of 0.15 nm, which effectively reduces the scattering loss in a waveguide. The growth of the strained-layer superlattice augments the nonlinear coupling coefficient kappa by utilizing the piezoelectric field in the transverse quasi-phase matching SHG device.
Authors
- Tomoyuki Tanikawa (ORCID: https://orcid.org/0000-0003-0148-9701)
- Ryuji Katayama (ORCID: https://orcid.org/0000-0002-7897-3393)
- Masahiro Uemukai
- Hideto Miyake
- Hiroto Honda (ORCID: https://orcid.org/0009-0000-8554-7598)
- Ryosuke Noro
- Kanako Shojiki (ORCID: https://orcid.org/0000-0003-0781-7016)
- Shahzeb Malik
- Masaaki Ito
Institutions
- Mie University (JP)
- Kyoto University (JP)
- Quantum (Australia) (AU)
- Spintronics Research Network of Japan (JP)
- Graduate School USA (US)
Publication Details
- Journal
- Crystal Growth & Design
- Published
- 2025-05-07
- DOI
- https://doi.org/10.1021/acs.cgd.4c01325
- Citations
- 2
- Primary Topic
- GaN-based semiconductor devices and materials
- Type
- article
- Field-Weighted Citation Impact
- 2.52
Funders
- Japan Society for the Promotion of Science