Magnetic Field Control of Liquid Crystal-Enabled Colloid Electrophoresis

Microswimmers are key for unveiling new physical phenomena underlying their propulsion, especially when driven inside complex fluids. Liquid crystals are anisotropic complex fluids that feature long-range orientational order. The propulsion of non-charged dielectric particles can be accomplished in these systems by breaking the particles’ fore-aft symmetry thanks to anisotropies in the conductivity and dielectric permittivity parameters of the liquid crystal. Under the application of an AC electric field, asymmetric osmotic flows are generated to propel non-spherical particles, whose direction of motion depends on the orientational order of the liquid crystal molecules around the inclusions. This means that, by controlling the LC orientation, one will be able to steer driven colloidal inclusions. In this experimental work, we show that a homogeneous magnetic field that is able to control the orientation of the liquid crystal molecules also allows us to determine the direction of motion of driven particles without significant changes in the propulsion mechanism. Additionally, we show that a radial configuration of the magnetic field lines can be used to generate topological defects in the liquid crystal orientational field that attract colloidal particles, leading to their clustering as rotating mills. The generated clusters were tested to study the collective motion of particles, suggesting the presence of particle–particle interactions.