Edge-Mediated Magnetic Domain Rearrangement in van der Waals Magnet Fe<sub>3</sub>GaTe<sub>2</sub>

The emergence of van der Waals (vdW) magnets has opened new frontiers for investigation of 2-dimensional magnetism and application of spintronic memories. However, as the system approached the nanoscale, the edge effect significantly enhanced, posing critical challenges in understanding edge-mediated modifications of magnetic behavior, such as the nanoscale magnetic domain. Here, we employ magnetic force microscopy to systematically investigate edge-mediated magnetic domain rearrangement in Fe<sub>3</sub>GaTe<sub>2</sub> flakes. By performing thermal treatment, we observed a distinct transition from labyrinthine to edge-localized stripe domains perpendicular to the flake edges. Furthermore, we reveal a competition and stabilization between size effect and edge effect by investigating thickness-dependent variation in the length of stripe domains and indicate that such an edge effect suppresses the formation of skyrmions. These findings not only elucidate the critical role of the edge effect in governing the domain morphology of vdW magnets but also provide insights for designing edge-mediated nanostructures in next-generation spintronic devices.

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Publication Details

Journal
Nano Letters
Published
2025-05-06
DOI
https://doi.org/10.1021/acs.nanolett.5c01181
Citations
1
Primary Topic
Inorganic Chemistry and Materials
Type
article
Field-Weighted Citation Impact
0.54
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Edge-Mediated Magnetic Domain Rearrangement in van der Waals Magnet Fe3GaTe2

Jiawang Hong, Boyuan Huang, Shuaizhao Jin, Tian‐Long Xia et al.
1 citations
Nano Letters
Inorganic Chemistry and Materials
0.54
article

Edge-Mediated Magnetic Domain Rearrangement in van der Waals Magnet Fe3GaTe2

Jiawang Hong, Boyuan Huang, Shuaizhao Jin, Tian‐Long Xia, Xueyun Wang, Baijun Gu, Yujia Liu, Xiangping Zhang, Yi‐Ting Wang, Yichong Chen
article en
1 citations

Abstract

The emergence of van der Waals (vdW) magnets has opened new frontiers for investigation of 2-dimensional magnetism and application of spintronic memories. However, as the system approached the nanoscale, the edge effect significantly enhanced, posing critical challenges in understanding edge-mediated modifications of magnetic behavior, such as the nanoscale magnetic domain. Here, we employ magnetic force microscopy to systematically investigate edge-mediated magnetic domain rearrangement in Fe<sub>3</sub>GaTe<sub>2</sub> flakes. By performing thermal treatment, we observed a distinct transition from labyrinthine to edge-localized stripe domains perpendicular to the flake edges. Furthermore, we reveal a competition and stabilization between size effect and edge effect by investigating thickness-dependent variation in the length of stripe domains and indicate that such an edge effect suppresses the formation of skyrmions. These findings not only elucidate the critical role of the edge effect in governing the domain morphology of vdW magnets but also provide insights for designing edge-mediated nanostructures in next-generation spintronic devices.

Nano LettersVol. 25(19)
Beijing Institute of Technology (CN), Southern University of Science and Technology (CN), Renmin University of China (CN)
Openalex Percentile: Top 37%
Inorganic Chemistry and Materials
0.54
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Edge-Mediated Magnetic Domain Rearrangement in van der Waals Magnet Fe<sub>3</sub>GaTe<sub>2</sub> — Jiawang Hong, Boyuan Huang, et al. · Nano Letters (2025) | TGRS Research Map | TGRS