Dual-Wavelength Operation at 607 nm and 640 nm with the Same Threshold and Slope Efficiency in Pr3+:LiLuF4 Crystal

A dual-wavelength (DW) Pr3+:LiLuF4 (Pr:LLF) laser with the same threshold and slope efficiency was achieved for the first time. We theoretically deduced the conditions for obtaining the same threshold and slope efficiency of the DW operation, and experimentally demonstrated the orange-red DW Pr:LLF laser by optimizing the output coupling transmittance and adjusting the rotation angle of the intracavity Lyot filter. A CW orange-red DW laser, pumped by a 10 W 479 nm frequency-doubled optically pumped semiconductor laser (2ω-OPSL), delivers combined outputs of 607 nm and 640 nm with a total power of 2.69 W. The orange and red wavelengths maintained balanced power output under each pump level. Furthermore, by a type-I critical phase-matched (CPM) β-BaB2O4 (BBO) crystal, a CW ultraviolet (UV) second harmonic generation (SHG) at 312 nm was also obtained through intracavity sum-frequency mixing (SFM) of the 607 nm and 640 nm fundamental beams, achieving a maximum power output of 812 mW.