On the drivers of ice nucleating particle diurnal variability in Eastern Mediterranean clouds
We report the drivers of spatiotemporal variability of ice nucleating particles (INPs) for mixed-phase orographic clouds (~-25 °C) in the Eastern Mediterranean. In the planetary boundary layer, pronounced INP diurnal periodicity is observed, which is mainly driven by biological (and to a lesser extent, dust) particles but not aerosols from biomass burning. The comparison of size-resolved and fluorescence-discriminated aerosol particle properties with INPs reveals the primary role of fluorescent bioaerosol. The presence of Saharan dust increases INPs during nighttime more than daytime, because of lower boundary layer height during nighttime which decreases the contribution of aerosols (including bioaerosols) from the boundary layer. INP diurnal periodicity is absent in the free troposphere, although levels are driven by the availability of bioaerosol and dust particles. Given the effective ice nucleation ability of bioaerosols and subsequent effects from ice multiplication at warm temperatures, the lack of such cycles in models points to important and overlooked drivers of cloud formation and precipitation in mountainous regions.
Authors
- Athanasios Nenes (ORCID: https://orcid.org/0000-0003-3873-9970)
- Stergios Vratolis (ORCID: https://orcid.org/0000-0002-2561-4653)
- Alexandros Papayannis (ORCID: https://orcid.org/0000-0002-5189-9381)
- Franziska Vogel (ORCID: https://orcid.org/0000-0002-9605-5684)
- Maria I. Gini (ORCID: https://orcid.org/0000-0001-8131-1211)
- Prodromos Fetfatzis (ORCID: https://orcid.org/0000-0002-9871-0259)
- Romanos Foskinis (ORCID: https://orcid.org/0000-0003-0221-3328)
- Kunfeng Gao (ORCID: https://orcid.org/0000-0001-9482-3857)
- Konstantinos Eleftheriadis (ORCID: https://orcid.org/0000-0003-2265-4905)
- Konstantinos Granakis (ORCID: https://orcid.org/0009-0007-8303-0545)
- Olga Zografou (ORCID: https://orcid.org/0000-0002-2889-2026)
- Ottmar Möhler (ORCID: https://orcid.org/0000-0002-7551-9814)
Institutions
- Karlsruhe Institute of Technology (DE)
- National Technical University of Athens (GR)
- National Centre of Scientific Research "Demokritos" (GR)
- ETH Zurich (CH)
- Institute for Biomedical Engineering (CH)
- Institute of Atmospheric Sciences and Climate (IT)
- École Polytechnique Fédérale de Lausanne (CH)
- Foundation for Research and Technology Hellas (GR)
Publication Details
- Journal
- npj Climate and Atmospheric Science
- Published
- 2025-05-05
- DOI
- https://doi.org/10.1038/s41612-024-00817-9
- Citations
- 3
- Primary Topic
- Atmospheric chemistry and aerosols
- Type
- article
- Field-Weighted Citation Impact
- 3.90
Funders
- National Science Foundation
- European Commission
- École Polytechnique Fédérale de Lausanne
- Schweizerischer Nationalfonds zur Förderung der Wissenschaftlichen Forschung
- National Technical University of Athens
- Horizon 2020 Framework Programme
- HORIZON EUROPE Framework Programme