Artificial Olfactory System Enabled by Ultralow Chemical Sensing Variations of 1D SnO <sub>2</sub> Nanoarchitectures

AI-assisted electronic nose systems often emphasize sensitivity-driven datasets, overlooking the comprehensive analysis of gaseous chemical attributes critical for precise gas identification. Conventional fabrication methods generate inconsistent datasets and focus primarily on improving classification accuracy through deep learning, neglecting the fundamental role of sensor material design. This study addresses these challenges by developing a highly reliable sensor platform to standardize gas sensing for deep learning applications. Specifically, 1D SnO<sub>2</sub> nanonetworks functionalized with Au and Pd nanocatalysts are fabricated via a systematic deposition process, enhancing gas diffusion and reaction kinetics. Stability improvements through controlled aging process reduce the coefficient of variation to below 5% across seven target gases: acetone, hydrogen, ethanol, carbon monoxide, propane, isoprene, and toluene. The platform exhibits exceptional deep learning performance, achieving over 99.5% classification accuracy using a residual network model, even in high-humidity environments (up to 80% relative humidity) and at parts-per-trillion detection limits. This study highlights the synergy between nanostructure engineering and AI, establishing a robust framework for next-generation bioinspired electronic nose systems with enhanced reliability and analytical capability.

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Publication Details

Journal
Advanced Science
Published
2025-05-03
DOI
https://doi.org/10.1002/advs.202501293
Citations
36
Primary Topic
Advanced Chemical Sensor Technologies
Type
article
Field-Weighted Citation Impact
24.27

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article

Artificial Olfactory System Enabled by Ultralow Chemical Sensing Variations of 1D SnO 2 Nanoarchitectures

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36 citations
Advanced Science
Advanced Chemical Sensor Technologies
24.27
article

Artificial Olfactory System Enabled by Ultralow Chemical Sensing Variations of 1D SnO 2 Nanoarchitectures

Zion Park, Ki Chang Kwon, Donghwi Cho, Gyu‐Li Kim, Young‐Seok Shim, Hyojung Kim, Jae‐Kwon Ko, Chil‐Hyoung Lee, Jeong‐O Lee, Kwangjae Lee, Tae Won Ha, Dongsu Kim, Yun‐Haeng Cho, S. T. Ro, Jae Han Chung, Jung Hwan Seo
article en
36 citations

Abstract

AI-assisted electronic nose systems often emphasize sensitivity-driven datasets, overlooking the comprehensive analysis of gaseous chemical attributes critical for precise gas identification. Conventional fabrication methods generate inconsistent datasets and focus primarily on improving classification accuracy through deep learning, neglecting the fundamental role of sensor material design. This study addresses these challenges by developing a highly reliable sensor platform to standardize gas sensing for deep learning applications. Specifically, 1D SnO<sub>2</sub> nanonetworks functionalized with Au and Pd nanocatalysts are fabricated via a systematic deposition process, enhancing gas diffusion and reaction kinetics. Stability improvements through controlled aging process reduce the coefficient of variation to below 5% across seven target gases: acetone, hydrogen, ethanol, carbon monoxide, propane, isoprene, and toluene. The platform exhibits exceptional deep learning performance, achieving over 99.5% classification accuracy using a residual network model, even in high-humidity environments (up to 80% relative humidity) and at parts-per-trillion detection limits. This study highlights the synergy between nanostructure engineering and AI, establishing a robust framework for next-generation bioinspired electronic nose systems with enhanced reliability and analytical capability.

Advanced ScienceVol. 12(25)
Sangmyung University (KR), Chungnam National University (KR), Korea Research Institute of Standards and Science (KR), Sejong University (KR), Korea University of Technology and Education (KR), Korea Research Institute of Chemical Technology (KR), Korea University of Science and Technology (KR), Korea Institute of Industrial Technology (KR), Hongik University (KR)
National Research Foundation, Ministry of Trade, Industry and Energy, Korea Research Institute of Chemical Technology, National Research Foundation of Korea, Ministry of Science and ICT, South Korea, Korea Evaluation Institute of Industrial Technology
Openalex Percentile: Top 0%
Advanced Chemical Sensor Technologies
24.27
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