Electric field-tuning plasmon and coupled plasmon–phonon modes in monolayer transition metal dichalcogenides

We theoretically investigate the electric field-tuning plasmons and plasmon–phonon couplings of two-dimensional (2D) transition metal dichalcogenides (TMDs), such as monolayer MoS2, under the consideration of spin–orbit coupling. It is revealed that the frequencies of plasmons and coupled plasmon-phonon modes originating from electron–electron and electron–phonon interactions can be effectively changed by using applied driving electric fields. Notably, these frequencies exhibit a decreasing trend with an increasing electric field. Moreover, the weak angular dependence of these modes suggests that the driving electric field does not induce significant anisotropy in the plasmon modes. The outcomes of this work demonstrate that the plasmon and coupled plasmon–phonon modes can be tuned not only by manipulating the electron density via the application of a gate voltage but also by tuning the applied driving electric field. These findings hold relevance for facilitating the application of 2D TMDs in optoelectronic devices.

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Publication Details

Journal
Journal of Applied Physics
Published
2025-05-02
DOI
https://doi.org/10.1063/5.0258357
Primary Topic
2D Materials and Applications
Type
article
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article

Electric field-tuning plasmon and coupled plasmon–phonon modes in monolayer transition metal dichalcogenides

H. M. Dong, Chengxiang Zhao, Fangwei Han, Haotong Wang et al.
Journal of Applied Physics
2D Materials and Applications
article

Electric field-tuning plasmon and coupled plasmon–phonon modes in monolayer transition metal dichalcogenides

H. M. Dong, Chengxiang Zhao, Fangwei Han, Haotong Wang, Wenjun Zhang
article en

Abstract

We theoretically investigate the electric field-tuning plasmons and plasmon–phonon couplings of two-dimensional (2D) transition metal dichalcogenides (TMDs), such as monolayer MoS2, under the consideration of spin–orbit coupling. It is revealed that the frequencies of plasmons and coupled plasmon-phonon modes originating from electron–electron and electron–phonon interactions can be effectively changed by using applied driving electric fields. Notably, these frequencies exhibit a decreasing trend with an increasing electric field. Moreover, the weak angular dependence of these modes suggests that the driving electric field does not induce significant anisotropy in the plasmon modes. The outcomes of this work demonstrate that the plasmon and coupled plasmon–phonon modes can be tuned not only by manipulating the electron density via the application of a gate voltage but also by tuning the applied driving electric field. These findings hold relevance for facilitating the application of 2D TMDs in optoelectronic devices.

Journal of Applied PhysicsVol. 137(17)
China University of Mining and Technology (CN), Jining Medical University (CN), Shanxi Normal University (CN)
Openalex Percentile: Top 94%
2D Materials and Applications
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