Doped organic thermoelectric short wavelength infrared detectors

Photon-based organic photodetector performance drops rapidly when going beyond near-infrared light detection due to nonradiative recombination. Here, we report on a device concept for infrared detection using organic thermoelectrics coupled to an infrared absorption film for heat generation. These short wavelength infrared (SWIR) detectors show an excellent area normalized responsivity of over 10<sup>9</sup> milliampere per watt per square meter at 1 V, two to three orders of magnitude higher than the conjugated polymer SWIR detector reported in the literature and typical organic photodetectors in the visible and near-infrared wavelength range. Moreover, the devices show a fast switch-on time with an estimated 3-decibel frequency of over 610 kilohertz, making the device suitable for a wide range of applications. However, the specific detectivity of the current device concept is limited to 10<sup>4</sup> Jones. We discuss strategies for improving the specific detectivities of these detectors with technology computer-aided design simulations.

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Publication Details

Journal
Science Advances
Published
2025-05-02
DOI
https://doi.org/10.1126/sciadv.adt0006
Citations
4
Primary Topic
Advanced Thermoelectric Materials and Devices
Type
article
Field-Weighted Citation Impact
2.07
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article

Doped organic thermoelectric short wavelength infrared detectors

Tiffany Wong, Johannes Benduhn, Karl Leo, Alexej Pashkin et al.
4 citations
Science Advances
Advanced Thermoelectric Materials and Devices
2.07
article

Doped organic thermoelectric short wavelength infrared detectors

Tiffany Wong, Johannes Benduhn, Karl Leo, Alexej Pashkin, Zongbao Zhang, Jakob Wolansky, Andrei Luferau, Louis Conrad Winkler, Hans Kleemann, Mohd Saif Shaikh, Yonder Berencén, Ghader Darbandy, Shu‐Jen Wang
article en
4 citations

Abstract

Photon-based organic photodetector performance drops rapidly when going beyond near-infrared light detection due to nonradiative recombination. Here, we report on a device concept for infrared detection using organic thermoelectrics coupled to an infrared absorption film for heat generation. These short wavelength infrared (SWIR) detectors show an excellent area normalized responsivity of over 10<sup>9</sup> milliampere per watt per square meter at 1 V, two to three orders of magnitude higher than the conjugated polymer SWIR detector reported in the literature and typical organic photodetectors in the visible and near-infrared wavelength range. Moreover, the devices show a fast switch-on time with an estimated 3-decibel frequency of over 610 kilohertz, making the device suitable for a wide range of applications. However, the specific detectivity of the current device concept is limited to 10<sup>4</sup> Jones. We discuss strategies for improving the specific detectivities of these detectors with technology computer-aided design simulations.

Science AdvancesVol. 11(18)
Hong Kong Baptist University (HK), Helmholtz-Zentrum Dresden-Rossendorf (DE), Technische Hochschule Mittelhessen (DE), Technische Universität Dresden (DE)
Affordable and clean energy
Openalex Percentile: Top 14%
Advanced Thermoelectric Materials and Devices
2.07
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