Substoichiometric silica in a multimaterial highly reflective coating

Abstract Gravitational-wave detectors impose exceptionally rigorous demands on optical coatings, which include high reflectivity, low thermal noise, low absorption, low scatter, and minimal defect counts. Simultaneously satisfying the thermal noise and absorption requirements is particularly challenging. One promising approach is to use three or more materials in a single coating. In this work we characterize such a multimaterial coating made using low index silica (SiO 2 ), high index tantala (Ta 2 O 5 ), and high index substoichiometric silica (SiO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mi>x</mml:mi> </mml:msub> </mml:mrow> </mml:math> ). We find that by using a multi-material structure, we achieve a more than 1000-fold reduction in optical absorption relative to a mirror made solely of SiO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mi>x</mml:mi> </mml:msub> </mml:mrow> </mml:math> and SiO 2 . Exploration of the SiO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mi>x</mml:mi> </mml:msub> </mml:mrow> </mml:math> deposition parameter space may allow for further optimization and we present one possible optimized coating design that may reduce coating thermal noise by 20% relative to the coatings used in current detectors.

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Publication Details

Journal
Classical and Quantum Gravity
Published
2025-05-01
DOI
https://doi.org/10.1088/1361-6382/add2c6
Citations
1
Primary Topic
Silicone and Siloxane Chemistry
Type
article
Field-Weighted Citation Impact
0.52

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article

Substoichiometric silica in a multimaterial highly reflective coating

G. Billingsley, Peter O’Brien, M. Evans, Liyuan Zhang et al.
1 citations
Classical and Quantum Gravity
Silicone and Siloxane Chemistry
0.52
article

Substoichiometric silica in a multimaterial highly reflective coating

G. Billingsley, Peter O’Brien, M. Evans, Liyuan Zhang, Nicholas Demos, Slawomir Gras
article en
1 citations

Abstract

Abstract Gravitational-wave detectors impose exceptionally rigorous demands on optical coatings, which include high reflectivity, low thermal noise, low absorption, low scatter, and minimal defect counts. Simultaneously satisfying the thermal noise and absorption requirements is particularly challenging. One promising approach is to use three or more materials in a single coating. In this work we characterize such a multimaterial coating made using low index silica (SiO 2 ), high index tantala (Ta 2 O 5 ), and high index substoichiometric silica (SiO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mi>x</mml:mi> </mml:msub> </mml:mrow> </mml:math> ). We find that by using a multi-material structure, we achieve a more than 1000-fold reduction in optical absorption relative to a mirror made solely of SiO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mi>x</mml:mi> </mml:msub> </mml:mrow> </mml:math> and SiO 2 . Exploration of the SiO <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" overflow="scroll"> <mml:mrow> <mml:msub> <mml:mrow/> <mml:mi>x</mml:mi> </mml:msub> </mml:mrow> </mml:math> deposition parameter space may allow for further optimization and we present one possible optimized coating design that may reduce coating thermal noise by 20% relative to the coatings used in current detectors.

Classical and Quantum GravityVol. 42(11)
California Institute of Technology (US), MIT Lincoln Laboratory (US), Massachusetts Institute of Technology (US)
National Science Foundation
Openalex Percentile: Top 39%
Silicone and Siloxane Chemistry
0.52
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Substoichiometric silica in a multimaterial highly reflective coating — G. Billingsley, Peter O’Brien, et al. · Classical and Quantum Gravity (2025) | TGRS Research Map | TGRS