Pyrolytic carbon membranes enabling novel low-energy photon sources

A compact non-radioactive ionization source is required for various detectors. A photoionization source utilizing a pure pyrolytic carbon membrane grown via chemical vapor deposition is developed and characterized. The efficient transmission of the carbon fluorescence line results in a high source efficiency at an acceleration voltage of 500 V. Comparative studies demonstrate that this source generates significantly higher ion currents at voltages below 2 kV compared to traditional configurations, including a carbon membrane coated with a 50 nm gold target and a 125 μm beryllium membrane coated with a 750 nm silver target. As a preliminary proof of principle, the photoionization source is evaluated using a field-switching ion mobility spectrometer. At an acceleration voltage of 500 V and an emission current of 5 μA, the pure carbon membrane configuration exhibits a twofold increase in the intensity of the ion peak compared to a tritium ionization source.

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Publication Details

Journal
Review of Scientific Instruments
Published
2025-05-01
DOI
https://doi.org/10.1063/5.0240264
Primary Topic
Mass Spectrometry Techniques and Applications
Type
article
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article

Pyrolytic carbon membranes enabling novel low-energy photon sources

Florian Herdl, Maximilian J. Kueddelsmann, Simon Edler, Felix Düsberg et al.
Review of Scientific Instruments
Mass Spectrometry Techniques and Applications
article

Pyrolytic carbon membranes enabling novel low-energy photon sources

Florian Herdl, Maximilian J. Kueddelsmann, Simon Edler, Felix Düsberg, Georg Stefan Duesberg, Andreas Pahlke, Stefan Zimmermann, Michael Bachmann, Natsuki Miyakawa, Andreas Schels, Erik Bunert, Max Kaschytza
article en

Abstract

A compact non-radioactive ionization source is required for various detectors. A photoionization source utilizing a pure pyrolytic carbon membrane grown via chemical vapor deposition is developed and characterized. The efficient transmission of the carbon fluorescence line results in a high source efficiency at an acceleration voltage of 500 V. Comparative studies demonstrate that this source generates significantly higher ion currents at voltages below 2 kV compared to traditional configurations, including a carbon membrane coated with a 50 nm gold target and a 125 μm beryllium membrane coated with a 750 nm silver target. As a preliminary proof of principle, the photoionization source is evaluated using a field-switching ion mobility spectrometer. At an acceleration voltage of 500 V and an emission current of 5 μA, the pure carbon membrane configuration exhibits a twofold increase in the intensity of the ion peak compared to a tritium ionization source.

Review of Scientific InstrumentsVol. 96(5)
Leibniz University Hannover (DE), Universität der Bundeswehr München (DE)
Affordable and clean energy
Openalex Percentile: Top 91%
Mass Spectrometry Techniques and Applications
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Pyrolytic carbon membranes enabling novel low-energy photon sources — Florian Herdl, Maximilian J. Kueddelsmann, et al. · Review of Scientific Instruments (2025) | TGRS Research Map | TGRS