2D-Supported Vertical MXenes for Ultrafast Filtering with Ultralow Inductance

Filtering supercapacitors (SCs) are promising for miniaturized power filter electronics due to their high capacitance and robust high-power performance. However, their adoption is limited by a poor low-frequency response in planar porous electrodes, causing mismatched operating frequencies and overheating risks. To address this, we develop MXene-based SCs using a novel vitamin C-assisted solution-thermal method to assemble Ti<sub>3</sub>C<sub>2</sub>T<sub><i>x</i></sub> MXenes into 2D-supported vertical structures, enhancing the dynamic response for linear filtering. These SCs achieve an ultrafast frequency response of 13.8 kHz at a phase angle of -45°, with electric inductance 1/2000 that of commercial aluminum electrolytic capacitors (AECs). They exhibit high areal and volumetric capacitances and effectively smooth random AC waveforms into stable DC signals. Their practicality is demonstrated by replacing bulky AECs and parallel capacitors in a Bluetooth audio amplifier, delivering wireless audio playback without tone quality loss and highlighting their transformative potential for next-generation electronics.

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Publication Details

Journal
Nano Letters
Published
2025-05-01
DOI
https://doi.org/10.1021/acs.nanolett.5c01020
Citations
7
Primary Topic
MXene and MAX Phase Materials
Type
article
Field-Weighted Citation Impact
3.62

Funders

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article

2D-Supported Vertical MXenes for Ultrafast Filtering with Ultralow Inductance

Shi Pu, Andreu Cabot, Yanting Xie, Zixing Wang et al.
7 citations
Nano Letters
MXene and MAX Phase Materials
3.62
article

2D-Supported Vertical MXenes for Ultrafast Filtering with Ultralow Inductance

Shi Pu, Andreu Cabot, Yanting Xie, Zixing Wang, Xiong Zhang, Haitao Zhang
article en
7 citations

Abstract

Filtering supercapacitors (SCs) are promising for miniaturized power filter electronics due to their high capacitance and robust high-power performance. However, their adoption is limited by a poor low-frequency response in planar porous electrodes, causing mismatched operating frequencies and overheating risks. To address this, we develop MXene-based SCs using a novel vitamin C-assisted solution-thermal method to assemble Ti<sub>3</sub>C<sub>2</sub>T<sub><i>x</i></sub> MXenes into 2D-supported vertical structures, enhancing the dynamic response for linear filtering. These SCs achieve an ultrafast frequency response of 13.8 kHz at a phase angle of -45°, with electric inductance 1/2000 that of commercial aluminum electrolytic capacitors (AECs). They exhibit high areal and volumetric capacitances and effectively smooth random AC waveforms into stable DC signals. Their practicality is demonstrated by replacing bulky AECs and parallel capacitors in a Bluetooth audio amplifier, delivering wireless audio playback without tone quality loss and highlighting their transformative potential for next-generation electronics.

Nano LettersVol. 25(19)
Institució Catalana de Recerca i Estudis Avançats (ES), J-Power (Japan) (JP), Hunan University (CN), Chinese Academy of Sciences (CN), Institut de Recerca en Energia de Catalunya (ES), Division of Materials Science and Engineering (AU), Chery Automobile (China) (CN), Southwest Jiaotong University (CN)
National Natural Science Foundation of China, China Scholarship Council, Department of Science and Technology of Sichuan Province, Natural Science Foundation of Sichuan Province
Openalex Percentile: Top 7%
MXene and MAX Phase Materials
3.62
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