Instrumental distortions in quantum optimal control

Quantum optimal control methods, such as gradient ascent pulse engineering (GRAPE), are used for precise manipulation of quantum states. Many of those methods were pioneered in magnetic resonance spectroscopy, where instrumental distortions are often negligible. However, that is not the case elsewhere: the usual jumble of cables, resonators, modulators, splitters, amplifiers, and filters can and would distort control signals. Those distortions may be non-linear; their inverse functions may be ill-defined and unstable; they may even vary from one day to the next and across the sample. Here we introduce the response-aware gradient ascent pulse engineering framework, which accounts for any cascade of differentiable distortions within the GRAPE optimization loop, does not require filter function inversion, and produces control sequences that are resilient to user-specified distortion cascades with user-specified parameter ensembles. The framework is implemented into the optimal control module supplied with versions 2.10 and later of the open-source Spinach library; the user needs to provide function handles returning the actions by the distortions and, optionally, parameter ensembles for those actions.

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Institutions

Publication Details

Journal
The Journal of Chemical Physics
Published
2025-04-25
DOI
https://doi.org/10.1063/5.0264092
Citations
6
Primary Topic
Spectroscopy and Quantum Chemical Studies
Type
article
Field-Weighted Citation Impact
7.48

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article

Instrumental distortions in quantum optimal control

Uluk Rasulov, Ilya Kuprov
6 citations
The Journal of Chemical Physics
Spectroscopy and Quantum Chemical Studies
7.48
article

Instrumental distortions in quantum optimal control

Uluk Rasulov, Ilya Kuprov
article en
6 citations

Abstract

Quantum optimal control methods, such as gradient ascent pulse engineering (GRAPE), are used for precise manipulation of quantum states. Many of those methods were pioneered in magnetic resonance spectroscopy, where instrumental distortions are often negligible. However, that is not the case elsewhere: the usual jumble of cables, resonators, modulators, splitters, amplifiers, and filters can and would distort control signals. Those distortions may be non-linear; their inverse functions may be ill-defined and unstable; they may even vary from one day to the next and across the sample. Here we introduce the response-aware gradient ascent pulse engineering framework, which accounts for any cascade of differentiable distortions within the GRAPE optimization loop, does not require filter function inversion, and produces control sequences that are resilient to user-specified distortion cascades with user-specified parameter ensembles. The framework is implemented into the optimal control module supplied with versions 2.10 and later of the open-source Spinach library; the user needs to provide function handles returning the actions by the distortions and, optionally, parameter ensembles for those actions.

The Journal of Chemical PhysicsVol. 162(16)
University of Southampton (GB), Weizmann Institute of Science (IL)
Nvidia, Weizmann Institute of Science, Engineering and Physical Sciences Research Council
Openalex Percentile: Top 3%
Spectroscopy and Quantum Chemical Studies
7.48
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