Photoelectron Spin Texture in Tunneling Ionization Induced by a Linearly Polarized Laser Pulse

The spin polarization of photoelectrons in tunneling ionization is investigated using numerical solutions of the time-dependent Schrödinger equation in companion with our analytic treatment via the spin-resolved strong-field approximation and classical trajectory Monte Carlo simulations. We demonstrate a nontrivial spin texture of photoelectrons in momentum space, exhibiting a vortex structure relative to the laser polarization axis. The momentum-resolved polarization stems from the emergence of spin-correlated quantum orbits in the continuum. For direct electrons in few-cycle pulses, the nonvanishing initial transverse velocity of the electron is responsible for the polarization, while in long pulses, the spin texture is essentially shaped by recollisions. Furthermore, the interference between direct and rescattering ionization leads to spin-polarized electron holography, offering an alternative method to extract atomic fine structural information.

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Publication Details

Journal
Physical Review Letters
Published
2025-04-25
DOI
https://doi.org/10.1103/physrevlett.134.163201
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
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article

Photoelectron Spin Texture in Tunneling Ionization Induced by a Linearly Polarized Laser Pulse

Karen Z. Hatsagortsyan, Pei-Lun He, Zhaohan Zhang, Christoph H. Keitel
Physical Review Letters
Laser-Matter Interactions and Applications
article

Photoelectron Spin Texture in Tunneling Ionization Induced by a Linearly Polarized Laser Pulse

Karen Z. Hatsagortsyan, Pei-Lun He, Zhaohan Zhang, Christoph H. Keitel
article en

Abstract

The spin polarization of photoelectrons in tunneling ionization is investigated using numerical solutions of the time-dependent Schrödinger equation in companion with our analytic treatment via the spin-resolved strong-field approximation and classical trajectory Monte Carlo simulations. We demonstrate a nontrivial spin texture of photoelectrons in momentum space, exhibiting a vortex structure relative to the laser polarization axis. The momentum-resolved polarization stems from the emergence of spin-correlated quantum orbits in the continuum. For direct electrons in few-cycle pulses, the nonvanishing initial transverse velocity of the electron is responsible for the polarization, while in long pulses, the spin texture is essentially shaped by recollisions. Furthermore, the interference between direct and rescattering ionization leads to spin-polarized electron holography, offering an alternative method to extract atomic fine structural information.

Physical Review LettersVol. 134(16)
Max Planck Institute for Nuclear Physics (DE)
Openalex Percentile: Top 93%
Laser-Matter Interactions and Applications
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Photoelectron Spin Texture in Tunneling Ionization Induced by a Linearly Polarized Laser Pulse — Karen Z. Hatsagortsyan, Pei-Lun He, et al. · Physical Review Letters (2025) | TGRS Research Map | TGRS