Robust Nodal Behavior in the Thermal Conductivity of Superconducting <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>UTe</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:m

The superconducting state of the heavy-fermion metal <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:msub><a:mrow><a:mi>UTe</a:mi></a:mrow><a:mrow><a:mn>2</a:mn></a:mrow></a:msub></a:mrow></a:math> has attracted considerable interest because of evidence of spin-triplet Cooper pairing and nontrivial topology. Progress on these questions requires identifying the presence or absence of nodes in the superconducting gap function and their dimension. In this article, we report a comprehensive study of the influence of disorder on the thermal transport in the superconducting state of <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:mrow><c:msub><c:mrow><c:mi>UTe</c:mi></c:mrow><c:mrow><c:mn>2</c:mn></c:mrow></c:msub></c:mrow></c:math>. Through detailed measurements of the magnetic-field dependence of the thermal conductivity in the zero-temperature limit, we obtain clear evidence of the presence of point nodes in the superconducting gap for all samples with transition temperatures ranging from 1.6 to 2.1 K obtained by different synthesis methods, including a refined self-flux method. This robustness implies the presence of symmetry-imposed nodes throughout the range studied, further confirmed via disorder-dependent calculations of the thermal transport in a model with a single pair of nodes. In addition to capturing the temperature dependence of the thermal conductivity up to <e:math xmlns:e="http://www.w3.org/1998/Math/MathML" display="inline"><e:msub><e:mi>T</e:mi><e:mi>c</e:mi></e:msub></e:math>, this model provides some information about the locations of the nodes, suggesting a <g:math xmlns:g="http://www.w3.org/1998/Math/MathML" display="inline"><g:msub><g:mi>B</g:mi><g:mrow><g:mn>1</g:mn><g:mi>u</g:mi></g:mrow></g:msub></g:math> or <i:math xmlns:i="http://www.w3.org/1998/Math/MathML" display="inline"><i:msub><i:mi>B</i:mi><i:mrow><i:mn>2</i:mn><i:mi>u</i:mi></i:mrow></i:msub></i:math> symmetry for the superconducting order parameter. Additionally, comparing the new, ultrahigh conductivity samples to older samples reveals a crossover between a low-field and a high-field regime at a single value of the magnetic field in all samples. In the high-field regime, the thermal conductivity at different disorder levels differs from each other by a simple offset, suggesting that some simple principle determines the physics of the mixed state, a fact which may illuminate trends observed in other clean nodal superconductors.

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Publication Details

Journal
Physical Review X
Published
2025-04-25
DOI
https://doi.org/10.1103/physrevx.15.021029
Citations
11
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
13.84

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article

Robust Nodal Behavior in the Thermal Conductivity of Superconducting <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>UTe</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:m

P. J. Hirschfeld, Johnpierre Paglione, Tristin Metz, Nicholas P. Butch et al.
11 citations
Physical Review X
Rare-earth and actinide compounds
13.84
article

Robust Nodal Behavior in the Thermal Conductivity of Superconducting <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML" display="inline"><mml:mrow><mml:msub><mml:mrow><mml:mi>UTe</mml:mi></mml:mrow><mml:mrow><mml:mn>2</mml:mn></mml:mrow></mml:m

P. J. Hirschfeld, Johnpierre Paglione, Tristin Metz, Nicholas P. Butch, Shanta Ranjan Saha, Corey E. Frank, Vivek Mishra, Ian Hayes
article en
11 citations

Abstract

The superconducting state of the heavy-fermion metal <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:msub><a:mrow><a:mi>UTe</a:mi></a:mrow><a:mrow><a:mn>2</a:mn></a:mrow></a:msub></a:mrow></a:math> has attracted considerable interest because of evidence of spin-triplet Cooper pairing and nontrivial topology. Progress on these questions requires identifying the presence or absence of nodes in the superconducting gap function and their dimension. In this article, we report a comprehensive study of the influence of disorder on the thermal transport in the superconducting state of <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:mrow><c:msub><c:mrow><c:mi>UTe</c:mi></c:mrow><c:mrow><c:mn>2</c:mn></c:mrow></c:msub></c:mrow></c:math>. Through detailed measurements of the magnetic-field dependence of the thermal conductivity in the zero-temperature limit, we obtain clear evidence of the presence of point nodes in the superconducting gap for all samples with transition temperatures ranging from 1.6 to 2.1 K obtained by different synthesis methods, including a refined self-flux method. This robustness implies the presence of symmetry-imposed nodes throughout the range studied, further confirmed via disorder-dependent calculations of the thermal transport in a model with a single pair of nodes. In addition to capturing the temperature dependence of the thermal conductivity up to <e:math xmlns:e="http://www.w3.org/1998/Math/MathML" display="inline"><e:msub><e:mi>T</e:mi><e:mi>c</e:mi></e:msub></e:math>, this model provides some information about the locations of the nodes, suggesting a <g:math xmlns:g="http://www.w3.org/1998/Math/MathML" display="inline"><g:msub><g:mi>B</g:mi><g:mrow><g:mn>1</g:mn><g:mi>u</g:mi></g:mrow></g:msub></g:math> or <i:math xmlns:i="http://www.w3.org/1998/Math/MathML" display="inline"><i:msub><i:mi>B</i:mi><i:mrow><i:mn>2</i:mn><i:mi>u</i:mi></i:mrow></i:msub></i:math> symmetry for the superconducting order parameter. Additionally, comparing the new, ultrahigh conductivity samples to older samples reveals a crossover between a low-field and a high-field regime at a single value of the magnetic field in all samples. In the high-field regime, the thermal conductivity at different disorder levels differs from each other by a simple offset, suggesting that some simple principle determines the physics of the mixed state, a fact which may illuminate trends observed in other clean nodal superconductors.

Physical Review XVol. 15(2)
Canadian Institute for Advanced Research (CA), Indian Institute of Technology Madras (IN), University of Florida (US), NIST Center for Neutron Research (US), University of Maryland, College Park (US)
National Science Foundation, U.S. Department of Energy, Gordon and Betty Moore Foundation, University of Maryland, National Institute of Standards and Technology, Division of Materials Research
Openalex Percentile: Top 1%
Rare-earth and actinide compounds
13.84
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