Electric-field-independent spin-orbit-coupling gap in <i>h</i>-BN-encapsulated bilayer graphene

The weak spin-orbit coupling (SOC) in bilayer graphene (BLG) is essential for encoding spin qubits while bringing technical challenges for extracting the opened small SOC gap ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in experiments. Moreover, in addition to the intrinsic Kane-Mele term, extrinsic mechanisms also contribute to SOC in BLG, especially under experimental conditions including encapsulation of BLG with hexagonal boron nitride (h-BN) and applying an external out-of-plane electric displacement field D. Although measurements of ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in h-BN-encapsulated BLG have been reported, the relatively large experimental variations and existing experimental controversy make it difficult to fully understand the physical origin of ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$. Here, we report a combined experimental and theoretical study on ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in h-BN-encapsulated BLG. We use an averaging method to extract ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in gate-defined single quantum dot devices. Under D fields as large as 0.57--0.90 V/nm, ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ \ensuremath{\approx} 53.4--61.8 $\text{\ensuremath{\mu}}$eV is obtained from two devices. Benchmarked with values reported at lower D field regime, our results support a D-field-independent ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$. This behavior is confirmed by our first-principles calculations, based on which ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ is found to be independent of D field, regardless of different h-BN/BLG/h-BN stacking configurations. Our calculations also suggest a weak proximity effect from h-BN, indicating that SOC in h-BN-encapsulated BLG is dominated by the intrinsic Kane-Mele mechanism. Our results offer insightful understanding of SOC in BLG, which benefits SOC engineering and spin manipulations in BLG.

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Publication Details

Journal
Physical Review Applied
Published
2025-04-24
DOI
https://doi.org/10.1103/physrevapplied.23.044053
Citations
6
Primary Topic
Graphene research and applications
Type
article
Field-Weighted Citation Impact
3.11

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article

Electric-field-independent spin-orbit-coupling gap in h-BN-encapsulated bilayer graphene

Ranran Cai, Gang Cao, Fang‐Ming Jing, Guo‐Quan Qin et al.
6 citations
Physical Review Applied
Graphene research and applications
3.11
article

Electric-field-independent spin-orbit-coupling gap in h-BN-encapsulated bilayer graphene

Ranran Cai, Gang Cao, Fang‐Ming Jing, Guo‐Quan Qin, Zhuo‐Zhi Zhang, Zhen-Xiong Shen, Xiang‐Xiang Song, Guo‐Ping Guo, Lixin He, Ting Lin, Wei-Kang Zhang
article en
6 citations

Abstract

The weak spin-orbit coupling (SOC) in bilayer graphene (BLG) is essential for encoding spin qubits while bringing technical challenges for extracting the opened small SOC gap ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in experiments. Moreover, in addition to the intrinsic Kane-Mele term, extrinsic mechanisms also contribute to SOC in BLG, especially under experimental conditions including encapsulation of BLG with hexagonal boron nitride (h-BN) and applying an external out-of-plane electric displacement field D. Although measurements of ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in h-BN-encapsulated BLG have been reported, the relatively large experimental variations and existing experimental controversy make it difficult to fully understand the physical origin of ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$. Here, we report a combined experimental and theoretical study on ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in h-BN-encapsulated BLG. We use an averaging method to extract ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ in gate-defined single quantum dot devices. Under D fields as large as 0.57--0.90 V/nm, ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ \ensuremath{\approx} 53.4--61.8 $\text{\ensuremath{\mu}}$eV is obtained from two devices. Benchmarked with values reported at lower D field regime, our results support a D-field-independent ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$. This behavior is confirmed by our first-principles calculations, based on which ${\mathrm{\ensuremath{\Delta}}}_{\mathrm{SO}}$ is found to be independent of D field, regardless of different h-BN/BLG/h-BN stacking configurations. Our calculations also suggest a weak proximity effect from h-BN, indicating that SOC in h-BN-encapsulated BLG is dominated by the intrinsic Kane-Mele mechanism. Our results offer insightful understanding of SOC in BLG, which benefits SOC engineering and spin manipulations in BLG.

Physical Review AppliedVol. 23(4)
University of Science and Technology of China (CN), National Science Centre (PL), Origin Quantum Computing Technology Company (China) (CN)
National Natural Science Foundation of China, China Postdoctoral Science Foundation, Natural Science Foundation of Jiangsu Province, University of Science and Technology of China
Openalex Percentile: Top 8%
Graphene research and applications
3.11
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