Photocurrent Nanoscopy of Quantum Hall Bulk

Understanding nanoscale electronic and thermal transport of two-dimensional (2D) electron systems in the quantum Hall regime, particularly in the bulk insulating state, poses considerable challenges. One of the primary difficulties arises from the presence of chiral edge channels, whose transport behavior obscures the investigation of the insulating bulk. Using near-field optical and photocurrent nanoscopy, we probe real-space variations of the optical and thermal dynamics of graphene in the quantum Hall regime without relying on complex sample or electrode geometries. Near the charge-neutrality point, we detect strong optical and photothermal signals from resonant inter-Landau-level (LL) magnetoexciton excitations between the zeroth and <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:mo>±</a:mo><a:mn>1</a:mn></a:mrow></a:math> st LLs, which gradually weaken with increasing doping due to Pauli blocking. Interestingly, at higher doping levels and full-integer LL fillings, photothermal signals reappear across the entire sample over an approximately <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:mrow><c:mn>10</c:mn><c:mtext>−</c:mtext><c:mrow><c:mi mathvariant="normal">μ</c:mi><c:mi mathvariant="normal">m</c:mi></c:mrow></c:mrow></c:math> scale, indicating unexpectedly long cooling lengths and nonlocal photothermal heating through the insulating bulk. This observation suggests that thermal conductivity persists for the localized states even as electronic transport is suppressed—a clear violation of the Wiedemann-Franz law. Our experiments provide novel insights into nanoscale thermal and electronic transport in incompressible 2D gases, highlighting the roles of magnetoexcitons and chiral edge states in the thermo-optoelectric dynamics of the Dirac quantum Hall state.

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Publication Details

Journal
Physical Review X
Published
2025-04-23
DOI
https://doi.org/10.1103/physrevx.15.021026
Citations
2
Primary Topic
Quantum and electron transport phenomena
Type
article
Field-Weighted Citation Impact
2.49

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article

Photocurrent Nanoscopy of Quantum Hall Bulk

Mengkun Liu, Yinan Dong, Lukas Wehmeier, Michael Dapolito et al.
2 citations
Physical Review X
Quantum and electron transport phenomena
2.49
article

Photocurrent Nanoscopy of Quantum Hall Bulk

Mengkun Liu, Yinan Dong, Lukas Wehmeier, Michael Dapolito, Zijian Zhou, D. N. Basov, Ran Jing, Bing Cheng, Xu Du, G. L. Carr, Qiang Li, Wenjun Zheng, Zengyi Du, Jiacheng Sun, Boyi Zhou, Shoujing Chen, Heng Wang
article en
2 citations

Abstract

Understanding nanoscale electronic and thermal transport of two-dimensional (2D) electron systems in the quantum Hall regime, particularly in the bulk insulating state, poses considerable challenges. One of the primary difficulties arises from the presence of chiral edge channels, whose transport behavior obscures the investigation of the insulating bulk. Using near-field optical and photocurrent nanoscopy, we probe real-space variations of the optical and thermal dynamics of graphene in the quantum Hall regime without relying on complex sample or electrode geometries. Near the charge-neutrality point, we detect strong optical and photothermal signals from resonant inter-Landau-level (LL) magnetoexciton excitations between the zeroth and <a:math xmlns:a="http://www.w3.org/1998/Math/MathML" display="inline"><a:mrow><a:mo>±</a:mo><a:mn>1</a:mn></a:mrow></a:math> st LLs, which gradually weaken with increasing doping due to Pauli blocking. Interestingly, at higher doping levels and full-integer LL fillings, photothermal signals reappear across the entire sample over an approximately <c:math xmlns:c="http://www.w3.org/1998/Math/MathML" display="inline"><c:mrow><c:mn>10</c:mn><c:mtext>−</c:mtext><c:mrow><c:mi mathvariant="normal">μ</c:mi><c:mi mathvariant="normal">m</c:mi></c:mrow></c:mrow></c:math> scale, indicating unexpectedly long cooling lengths and nonlocal photothermal heating through the insulating bulk. This observation suggests that thermal conductivity persists for the localized states even as electronic transport is suppressed—a clear violation of the Wiedemann-Franz law. Our experiments provide novel insights into nanoscale thermal and electronic transport in incompressible 2D gases, highlighting the roles of magnetoexcitons and chiral edge states in the thermo-optoelectric dynamics of the Dirac quantum Hall state.

Physical Review XVol. 15(2)
Brookhaven National Laboratory (US), Stony Brook University (US), Columbia University (US)
U.S. Department of Energy, Gordon and Betty Moore Foundation, Yale University, Nanyang Technological University, Stony Brook University, Office of Science, University of California, San Diego, Basic Energy Sciences, Energy Frontier Research Centers, Division of Materials Sciences and Engineering
Openalex Percentile: Top 12%
Quantum and electron transport phenomena
2.49
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