Gelatin-wax-based bigel System: Innovative research on a low-calorie fat substitute

In this study, we used beeswax and rice bran wax as oleogelators. We used gelatin as a hydrogelator for the hydrogels. Then, we checked the bigels' thermal, mechanical, rheological, and freeze-thaw properties with different mixes of hydrogel and oleogel. As the tests went on, it was found that when the ratio of hydrogel to oleogel was 6:4, the BG5 bigel had a water-oil bicontinuous phase. The Fourier transform infrared spectroscopy (FTIR) analysis indicated that the hydrogel and oleogel parts each had their own unique peaks. This pattern is similar to the lipid profile of butter. The storage modulus (G′) and loss modulus (G″) of the bigel changed in a way that wasn't linear as the hydrogel content went up. This indicated that the ratio of hydrogel to oleogel had a big effect on the bigel's elastic and viscous properties. Tests of freeze-thaw stability indicated that the oil holding capacity (OHC) went up significantly as the hydrogel content went up. Following three freeze-thaw cycles, the OHC values for BG2 to BG6 were 71.62 ± 1.03 %, 75.1 ± 0.36 %, 76.0 ± 0.02 %, 80.53 ± 1.85 %, and 99.60 ± 0.39 %. This study proposes a bigel preparation method with excellent structural and freeze–thaw stability, providing a new approach and technical support for the development of butter alternatives in low-fat food systems. • The bigel exhibits excellent freeze-thaw stability and oil retention capacity. • The hydrogel proportion has a complex effect on the elasticity of the bigel. • The bigel can combine the characteristics of both hydrogel and oleogel.

Authors

Publication Details

Journal
LWT
Published
2025-04-23
DOI
https://doi.org/10.1016/j.lwt.2025.117836
Citations
5
Primary Topic
Food Chemistry and Fat Analysis
Type
article
Field-Weighted Citation Impact
5.81

Funders

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article

Gelatin-wax-based bigel System: Innovative research on a low-calorie fat substitute

Juming Tang, Bin Li, Aolin Wu, Zhigang Hu et al.
5 citations
LWT
Food Chemistry and Fat Analysis
5.81
article

Gelatin-wax-based bigel System: Innovative research on a low-calorie fat substitute

Juming Tang, Bin Li, Aolin Wu, Zhigang Hu, Mengjing Zhou, Ying Wang, Jiawei Li
article en
5 citations

Abstract

In this study, we used beeswax and rice bran wax as oleogelators. We used gelatin as a hydrogelator for the hydrogels. Then, we checked the bigels' thermal, mechanical, rheological, and freeze-thaw properties with different mixes of hydrogel and oleogel. As the tests went on, it was found that when the ratio of hydrogel to oleogel was 6:4, the BG5 bigel had a water-oil bicontinuous phase. The Fourier transform infrared spectroscopy (FTIR) analysis indicated that the hydrogel and oleogel parts each had their own unique peaks. This pattern is similar to the lipid profile of butter. The storage modulus (G′) and loss modulus (G″) of the bigel changed in a way that wasn't linear as the hydrogel content went up. This indicated that the ratio of hydrogel to oleogel had a big effect on the bigel's elastic and viscous properties. Tests of freeze-thaw stability indicated that the oil holding capacity (OHC) went up significantly as the hydrogel content went up. Following three freeze-thaw cycles, the OHC values for BG2 to BG6 were 71.62 ± 1.03 %, 75.1 ± 0.36 %, 76.0 ± 0.02 %, 80.53 ± 1.85 %, and 99.60 ± 0.39 %. This study proposes a bigel preparation method with excellent structural and freeze–thaw stability, providing a new approach and technical support for the development of butter alternatives in low-fat food systems. • The bigel exhibits excellent freeze-thaw stability and oil retention capacity. • The hydrogel proportion has a complex effect on the elasticity of the bigel. • The bigel can combine the characteristics of both hydrogel and oleogel.

LWTVol. 224
Natural Science Foundation of Hubei Province, Wuhan Polytechnic University, Fundamental Research Funds for the Central Universities
Openalex Percentile: Top 5%
Food Chemistry and Fat Analysis
5.81
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Gelatin-wax-based bigel System: Innovative research on a low-calorie fat substitute — Juming Tang, Bin Li, et al. · LWT (2025) | TGRS Research Map | TGRS