Self-powered ultraviolet photodetector enabled by a quasi-n-p-n heterostructure of SnO2 colloidal quantum dots, p-GaN, and a two-dimensional electron gas at the AlGaN/GaN interface

Ultraviolet photodetectors (UV-PDs) are essential for a wide range of applications, yet their practical use is often limited by challenges such as low responsivity , high noise, and significant dark current , particularly in self-powered configurations. In this work, we present a self-powered UV photodetector based on SnO 2 colloidal quantum dots (CQDs) integrated with a p-GaN/AlGaN/GaN heterostructure . The device utilizes the built-in electric field at the SnO 2 /p-GaN interface to achieve self-powered operation and incorporates a quasi-n-p-n heterostructure formed between the SnO 2 CQDs (n-type), p-GaN (p-type), and the 2DEG (n-type) at the AlGaN/GaN interface to enhance carrier separation and transport, while minimizing dark current . The device demonstrates an ultra-low dark current of 370 fA in self-powered mode. At 255 nm and 340 nm, it achieves responsivities of 90.3 mA W −1 and 321.1 mA W −1 , respectively, with specific detectivities of 4.32 × 10 12 and 1.58 × 10 13 Jones. The photodetector exhibits strong broadband UV sensitivity spanning from 250 nm to 370 nm and sharp selectivity , with R 255 /R 400 and R 340 /R 400 ratios exceeding 10 4 . This work highlights the potential of SnO 2 /p-GaN/AlGaN/GaN-based self-powered UV photodetectors for advanced applications in UV communication, environmental monitoring, and defense systems, offering a platform for efficient and portable photonic devices . • Ultra-low dark current of 370 fA enables high-SNR self-powered UV detection. • Quasi-n-p-n heterostructure boosts carrier separation and suppresses recombination. • SnO 2 CQDs extend UV detection range from 250 to 370 nm with high responsivity. • Device shows visible rejection ratio over 10 4 with strong UV selectivity . • Fast response and broadband detection suitable for imaging and communication.

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Publication Details

Journal
Nano Energy
Published
2025-04-23
DOI
https://doi.org/10.1016/j.nanoen.2025.111047
Citations
6
Primary Topic
Ga2O3 and related materials
Type
article
Field-Weighted Citation Impact
2.56

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article

Self-powered ultraviolet photodetector enabled by a quasi-n-p-n heterostructure of SnO2 colloidal quantum dots, p-GaN, and a two-dimensional electron gas at the AlGaN/GaN interface

Xian Wu, Jing Wang, Tian‐Ling Ren, Sen Gao et al.
6 citations
Nano Energy
Ga2O3 and related materials
2.56
article

Self-powered ultraviolet photodetector enabled by a quasi-n-p-n heterostructure of SnO2 colloidal quantum dots, p-GaN, and a two-dimensional electron gas at the AlGaN/GaN interface

Xian Wu, Jing Wang, Tian‐Ling Ren, Sen Gao, Renrong Liang, Lei Xiao
article en
6 citations

Abstract

Ultraviolet photodetectors (UV-PDs) are essential for a wide range of applications, yet their practical use is often limited by challenges such as low responsivity , high noise, and significant dark current , particularly in self-powered configurations. In this work, we present a self-powered UV photodetector based on SnO 2 colloidal quantum dots (CQDs) integrated with a p-GaN/AlGaN/GaN heterostructure . The device utilizes the built-in electric field at the SnO 2 /p-GaN interface to achieve self-powered operation and incorporates a quasi-n-p-n heterostructure formed between the SnO 2 CQDs (n-type), p-GaN (p-type), and the 2DEG (n-type) at the AlGaN/GaN interface to enhance carrier separation and transport, while minimizing dark current . The device demonstrates an ultra-low dark current of 370 fA in self-powered mode. At 255 nm and 340 nm, it achieves responsivities of 90.3 mA W −1 and 321.1 mA W −1 , respectively, with specific detectivities of 4.32 × 10 12 and 1.58 × 10 13 Jones. The photodetector exhibits strong broadband UV sensitivity spanning from 250 nm to 370 nm and sharp selectivity , with R 255 /R 400 and R 340 /R 400 ratios exceeding 10 4 . This work highlights the potential of SnO 2 /p-GaN/AlGaN/GaN-based self-powered UV photodetectors for advanced applications in UV communication, environmental monitoring, and defense systems, offering a platform for efficient and portable photonic devices . • Ultra-low dark current of 370 fA enables high-SNR self-powered UV detection. • Quasi-n-p-n heterostructure boosts carrier separation and suppresses recombination. • SnO 2 CQDs extend UV detection range from 250 to 370 nm with high responsivity. • Device shows visible rejection ratio over 10 4 with strong UV selectivity . • Fast response and broadband detection suitable for imaging and communication.

Nano EnergyVol. 140
Tsinghua University (CN)
National Natural Science Foundation of China, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 10%
Ga2O3 and related materials
2.56
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