Sub-2 Kelvin Characterization of Nitrogen-Vacancy Centers in Silicon Carbide Nanopillars

The development of efficient quantum communication technologies depends on the innovation in multiple layers of its implementation, a challenge we address from the fundamental properties of the physical system at the nanoscale to the instrumentation level at the macroscale. We select a promising near-infrared quantum emitter, the nitrogen-vacancy (NV) center in 4H-SiC, and integrate it, at an ensemble level, with nanopillar structures that enhance photon collection efficiency into an objective lens. Moreover, changes in collection efficiency in pillars compared to bulk can serve as indicators of color center orientation in the lattice. To characterize NV center properties at the unprecedented sub-2 K temperatures, we incorporate compatible superconducting nanowire single photon detectors inside the chamber of an optical cryostat and create the ICECAP, the Integrated Cryogenic system for Emission, Collection And Photon detection. ICECAP measurements show no significant line-width broadening of NV ensemble emission and up to 14-fold enhancement in collected emission. With additional filtering, we measure emitter lifetimes of NV centers in a basal (<i>hk</i>) and axial (<i>kk</i>) orientation, unveiling their cryogenic values of 2.2 and 2.8 ns.

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Publication Details

Journal
ACS Photonics
Published
2025-04-22
DOI
https://doi.org/10.1021/acsphotonics.5c00096
Citations
5
Primary Topic
Diamond and Carbon-based Materials Research
Type
article
Field-Weighted Citation Impact
2.59

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article

Sub-2 Kelvin Characterization of Nitrogen-Vacancy Centers in Silicon Carbide Nanopillars

S. Virasawmy, Victoria A. Norman, A. H. Rubin, Scott Dhuey et al.
5 citations
ACS Photonics
Diamond and Carbon-based Materials Research
2.59
article

Sub-2 Kelvin Characterization of Nitrogen-Vacancy Centers in Silicon Carbide Nanopillars

S. Virasawmy, Victoria A. Norman, A. H. Rubin, Scott Dhuey, Sridhar Majety, Pranta Saha, Marina Radulaski, Bradi Palomarez, Pietra B. Curro, Liang Li, Jeanette Simo, N. González
article en
5 citations

Abstract

The development of efficient quantum communication technologies depends on the innovation in multiple layers of its implementation, a challenge we address from the fundamental properties of the physical system at the nanoscale to the instrumentation level at the macroscale. We select a promising near-infrared quantum emitter, the nitrogen-vacancy (NV) center in 4H-SiC, and integrate it, at an ensemble level, with nanopillar structures that enhance photon collection efficiency into an objective lens. Moreover, changes in collection efficiency in pillars compared to bulk can serve as indicators of color center orientation in the lattice. To characterize NV center properties at the unprecedented sub-2 K temperatures, we incorporate compatible superconducting nanowire single photon detectors inside the chamber of an optical cryostat and create the ICECAP, the Integrated Cryogenic system for Emission, Collection And Photon detection. ICECAP measurements show no significant line-width broadening of NV ensemble emission and up to 14-fold enhancement in collected emission. With additional filtering, we measure emitter lifetimes of NV centers in a basal (<i>hk</i>) and axial (<i>kk</i>) orientation, unveiling their cryogenic values of 2.2 and 2.8 ns.

ACS PhotonicsVol. 12(5)
Lawrence Berkeley National Laboratory (US), Santa Clara University (US), University of California, Davis (US)
Division of Physics, Division of Electrical, Communications and Cyber Systems, Basic Energy Sciences
Openalex Percentile: Top 11%
Diamond and Carbon-based Materials Research
2.59
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