HM-C21: A three-dimensional carbon with abundant p-electron-induced magnetic states for spintronics
Due to their long-distance spin transport and long spin lifetime, p-electron-induced spintronic materials have been attracting increasing attention. As the most common d-electron-free elements, carbon allotropes present many excellent properties. However, pure three-dimensional carbon spintronics material has not been reported so far. Here, we proposed a superhard (HV = 60 GPa) carbon material named half-metal (HM)-C21, which presents multi-stable magnetic states and unexpected properties, such as those of half-metal, half-semiconductor, bipolar magnetic semiconductor, and asymmetric antiferromagnetic semiconductors. The mechanical, dynamical, and thermodynamical stabilities of HM-C21 are confirmed. Moreover, HM-C21 is considered to be a promising candidate for an unidentified cubic-form carbon reported in previous experiments. Hence, the present work holds great promise for discovering spintronic materials in pure three-dimensional carbon.
Authors
- Mingqing Liao (ORCID: https://orcid.org/0000-0001-9765-3400)
- Fei Zhou (ORCID: https://orcid.org/0000-0002-5389-1009)
- Jintong Guan (ORCID: https://orcid.org/0000-0003-4354-6815)
- Hao Jiang (ORCID: https://orcid.org/0000-0002-4388-6548)
- Yuehua Wang
- Fengjiang Wang (ORCID: https://orcid.org/0000-0002-0613-8129)
- Chenggang Wu (ORCID: https://orcid.org/0009-0008-0103-0873)
- Nan Qu (ORCID: https://orcid.org/0000-0002-9226-0648)
- Jiayu Zhang (ORCID: https://orcid.org/0000-0002-8180-5796)
- Danni Yang (ORCID: https://orcid.org/0000-0002-6993-0543)
- Junjie Zhao (ORCID: https://orcid.org/0009-0004-3334-6283)
Institutions
- Jiangsu University (CN)
- Southwest University of Science and Technology (CN)
- Harbin Institute of Technology (CN)
- Lanzhou University of Technology (CN)
- Jiangsu University of Science and Technology (CN)
- Division of Materials Science and Engineering (AU)
Publication Details
- Journal
- Applied Physics Letters
- Published
- 2025-04-21
- DOI
- https://doi.org/10.1063/5.0247503
- Citations
- 2
- Primary Topic
- Boron and Carbon Nanomaterials Research
- Type
- article
- Field-Weighted Citation Impact
- 1.04
Funders
- Natural Science Foundation of Jiangsu Province