Asymmetric simple exclusion process with concerted hopping
An important mechanism enabling fast ion diffusion in solid electrolytes is considered to be the significant lowering of the activation barrier when two or more ion particles hop simultaneously between sites, i.e., concerted migration, compared to single-ion hopping. In this study we incorporate a mechanism of simultaneous particle hopping into the asymmetric simple exclusion process, which is an archetypal model for many-particle transportation phenomena, and investigate its impact on particle transport properties. In our model, reflecting ion dynamics, the hopping rates are controlled by the activation energy, inverse temperature, and strength of an external driving field. We first construct an exact solution that describes the steady state of the proposed model. By using this solution, we find that concerted migration substantially increases the particle current and induces a shift of the peak in the fundamental diagram, i.e., the density-current relationship. We also show the presence of a critical temperature that maximizes the current. Additionally, we discuss the implications within parameter regions corresponding to actual materials.
Authors
- Yasunobu Ando (ORCID: https://orcid.org/0000-0003-3702-034X)
- K. Kihara
- Katsuhiro Nishinari (ORCID: https://orcid.org/0000-0003-3069-1757)
- Takahiro Ezaki (ORCID: https://orcid.org/0000-0003-4175-3028)
Institutions
- Shanghai Institute for Science of Science (CN)
- Institute of Science Tokyo (JP)
- The University of Tokyo (JP)
Publication Details
- Journal
- Physical Review Research
- Published
- 2025-04-21
- DOI
- https://doi.org/10.1103/physrevresearch.7.023068
- Citations
- 1
- Primary Topic
- Stochastic processes and statistical mechanics
- Type
- article
- Field-Weighted Citation Impact
- 3.69
Funders
- Japan Society for the Promotion of Science