Enhanced room-temperature stimulated emission in a WS<sub>2</sub>-based plasmonic heterostructure

Transition metal dichalcogenides (TMDCs) offer tremendous prospects in the field of ultimate nanolasers due to their large exciton binding energies and atomic-scale thickness. The integration of TMDCs and plasmonic systems provides great potential for further miniaturization of device footprints. However, limitations in plasmon–exciton interactions and losses in plasmonic structures have restricted advancements in device performance. This study introduces a heterostructure that combines pretreated WS 2 with Au microplate gratings, which provides a low-loss platform that reduces non-radiative recombination. By optimizing the structural parameters, we enhance the coupling between excitons and surface plasmon polaritons (SPPs), effectively improving the coupling strength approximately threefold, which tends toward the strong coupling region. Furthermore, by utilizing the plasmonic bound states in the continuum (BIC), we achieve room-temperature stimulated emission amplification with nanosecond-pulsed pump powers exceeding 2.59 MW/cm 2 . Our findings provide a practical strategy for developing on-chip coherent light sources based on monolayer two-dimensional (2D) semiconductor–plasmonic structures, offering valuable insights into the interactions between plasmons and excitons.

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Publication Details

Journal
Optics Letters
Published
2025-04-21
DOI
https://doi.org/10.1364/ol.562321
Citations
1
Primary Topic
Gold and Silver Nanoparticles Synthesis and Applications
Type
article
Field-Weighted Citation Impact
0.43
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Enhanced room-temperature stimulated emission in a WS2-based plasmonic heterostructure

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Optics Letters
Gold and Silver Nanoparticles Synthesis and Applications
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article

Enhanced room-temperature stimulated emission in a WS2-based plasmonic heterostructure

Weiping Wu, Zong-Ru Yang, Zexian Chen, Tong Zhang, Xiaoman Li, Zhen-Zhi Hu, Yuanjun Song, Huan‐Li Zhou, Dan Su, Zhao-Guo Liu, Xiaoyang Zhang, K. Foua Bi
article en
1 citations

Abstract

Transition metal dichalcogenides (TMDCs) offer tremendous prospects in the field of ultimate nanolasers due to their large exciton binding energies and atomic-scale thickness. The integration of TMDCs and plasmonic systems provides great potential for further miniaturization of device footprints. However, limitations in plasmon–exciton interactions and losses in plasmonic structures have restricted advancements in device performance. This study introduces a heterostructure that combines pretreated WS 2 with Au microplate gratings, which provides a low-loss platform that reduces non-radiative recombination. By optimizing the structural parameters, we enhance the coupling between excitons and surface plasmon polaritons (SPPs), effectively improving the coupling strength approximately threefold, which tends toward the strong coupling region. Furthermore, by utilizing the plasmonic bound states in the continuum (BIC), we achieve room-temperature stimulated emission amplification with nanosecond-pulsed pump powers exceeding 2.59 MW/cm 2 . Our findings provide a practical strategy for developing on-chip coherent light sources based on monolayer two-dimensional (2D) semiconductor–plasmonic structures, offering valuable insights into the interactions between plasmons and excitons.

Optics LettersVol. 50(10)
Chinese Academy of Sciences (CN)
Affordable and clean energy
Openalex Percentile: Top 43%
Gold and Silver Nanoparticles Synthesis and Applications
0.43
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