High-Performance Oxide Thin-Film Transistors with Atomic Layer Deposition-Grown HfO<sub>2</sub>/BeO Hetero-Dielectric
Atomic layer deposition-grown beryllium oxide (BeO) is gaining attention as a dielectric material that can minimize device power consumption because of its high dielectric constant, high thermal conductivity, and low leakage current enabled by its wide bandgap energy. In this study, the impact of BeO dielectrics on InSnZnO (ITZO) thin-film transistors (TFTs) was investigated, revealing that adding a hafnium dioxide (HfO<sub>2</sub>) layer can enhance electrical performance and bias stress reliability. Time-of-flight secondary-ion mass spectrometry and X-ray photoelectron spectroscopy confirmed that the single-BeO dielectric-based ITZO TFTs exhibited a low mobility of 27.6 cm<sup>2</sup>/V·s due to Be migration and demonstrated abnormal threshold voltage (<i>V</i><sub>TH</sub>) shifts under bias stress. Conversely, the HfO<sub>2</sub> 20 nm/BeO hetero-dielectric ITZO TFTs exhibited a high mobility of 76.6 cm<sup>2</sup>/V·s and enhanced abnormal <i>V</i><sub>TH</sub> shift characteristics. Therefore, these results demonstrate that our high-performance HfO<sub>2</sub>/BeO hetero-dielectric-based ITZO TFTs could be utilized in back-end-of-line devices for monolithic three-dimensional memory technologies.
Authors
- Min‐Kyu Song (ORCID: https://orcid.org/0000-0002-9233-9356)
- Yoonseo Jang
- Jang‐Yeon Kwon (ORCID: https://orcid.org/0000-0002-5231-8307)
- Wooho Ham (ORCID: https://orcid.org/0009-0000-0777-8163)
- Jungwoo Oh (ORCID: https://orcid.org/0000-0002-6065-6250)
- Dohwan Jung
- Sein Lee (ORCID: https://orcid.org/0000-0002-6715-2389)
- Junseo Lee (ORCID: https://orcid.org/0009-0007-7850-7871)
- Jae‐Hoon Han (ORCID: https://orcid.org/0000-0003-3575-9140)
- Jonghyun Bae
- Prakash R. Sultane (ORCID: https://orcid.org/0000-0001-9862-7589)
- Jeong-Min Park (ORCID: https://orcid.org/0000-0003-3534-7947)
- Christopher W. Bielawski
- Kyunghwan Kim (ORCID: https://orcid.org/0009-0003-7031-6465)
Institutions
- Yonsei University (KR)
- Institute for Basic Science (KR)
- Intelligent Health (United Kingdom) (GB)
- Ulsan National Institute of Science and Technology (KR)
- Korea Institute of Science and Technology (KR)
- Massachusetts Institute of Technology (US)
Publication Details
- Journal
- Nano Letters
- Published
- 2025-04-21
- DOI
- https://doi.org/10.1021/acs.nanolett.5c00552
- Citations
- 5
- Primary Topic
- Semiconductor materials and devices
- Type
- article
- Field-Weighted Citation Impact
- 3.65
Funders
- National Research Foundation of Korea
- Institute for Basic Science