β-Ga2O3:Cr nanowires with optical microcavities for determining local heating induced by x-ray nanobeams
This study explores the x-ray excited optical luminescence (XEOL) of optical microcavities fabricated in β-Ga2O3:Cr nanowires (NWs). XEOL measurements reveal prominent luminescence bands in the near ultraviolet-blue (NUV-B) and in the red-near infrared (R-NIR) spectral regions. The NUV-B emission originates from β-Ga2O3 defects, while the R-NIR band is attributed to Cr3+ intraionic transitions. Both spectral regions exhibit sharp resonances, which are analyzed as Fabry–Pérot and whispering gallery mode resonances. Exposure to x-ray nanobeam induces a redshift of the sharp R-NIR peaks, attributed to local temperature increase in the NWs caused by x-ray absorption. The influence of this temperature rise on the NUV-B peaks is also evaluated. In addition, the local temperature increase due to x-ray absorption is estimated through COMSOL finite-difference time-domain simulations, incorporating the material’s physical and thermal properties. This work demonstrates the application of β-Ga2O3:Cr optical microcavities as luminescence-based nanothermometers to probe the localized effects of x-ray nanobeam irradiation.
Authors
- Jaime Dolado (ORCID: https://orcid.org/0000-0003-4183-2834)
- Gema Martínez‐Criado (ORCID: https://orcid.org/0000-0002-4503-9385)
- M.L. Nó (ORCID: https://orcid.org/0000-0003-3606-3700)
- Beatriz Rodríguez (ORCID: https://orcid.org/0000-0003-1744-1972)
- Bianchi Méndez (ORCID: https://orcid.org/0000-0002-6289-7437)
- Pedro Hidalgo (ORCID: https://orcid.org/0000-0001-5207-9660)
- Emilio Nogales (ORCID: https://orcid.org/0000-0003-3376-6320)
- J. San Juán (ORCID: https://orcid.org/0000-0002-5797-0687)
- Manuel Alonso‐Orts (ORCID: https://orcid.org/0000-0001-5043-4921)
- Daniel Carrasco (ORCID: https://orcid.org/0000-0002-7936-8187)
- Paula Pérez‐Peinado
Institutions
- Universidad Complutense de Madrid (ES)
- University of the Basque Country (ES)
- University of Bremen (DE)
- European Synchrotron Radiation Facility (FR)
- Instituto de Ciencia de Materiales de Madrid (ES)
Publication Details
- Journal
- APL Materials
- Published
- 2025-04-01
- DOI
- https://doi.org/10.1063/5.0261501
- Citations
- 1
- Primary Topic
- Ga2O3 and related materials
- Type
- article
- Field-Weighted Citation Impact
- 0.43
Funders
- Comunidad de Madrid
- Deutsche Forschungsgemeinschaft
- European Synchrotron Radiation Facility
- Ministerio de Ciencia e Innovación
- Universität Bremen
- Air Force Office of Scientific Research