β-Ga2O3:Cr nanowires with optical microcavities for determining local heating induced by x-ray nanobeams

This study explores the x-ray excited optical luminescence (XEOL) of optical microcavities fabricated in β-Ga2O3:Cr nanowires (NWs). XEOL measurements reveal prominent luminescence bands in the near ultraviolet-blue (NUV-B) and in the red-near infrared (R-NIR) spectral regions. The NUV-B emission originates from β-Ga2O3 defects, while the R-NIR band is attributed to Cr3+ intraionic transitions. Both spectral regions exhibit sharp resonances, which are analyzed as Fabry–Pérot and whispering gallery mode resonances. Exposure to x-ray nanobeam induces a redshift of the sharp R-NIR peaks, attributed to local temperature increase in the NWs caused by x-ray absorption. The influence of this temperature rise on the NUV-B peaks is also evaluated. In addition, the local temperature increase due to x-ray absorption is estimated through COMSOL finite-difference time-domain simulations, incorporating the material’s physical and thermal properties. This work demonstrates the application of β-Ga2O3:Cr optical microcavities as luminescence-based nanothermometers to probe the localized effects of x-ray nanobeam irradiation.

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Publication Details

Journal
APL Materials
Published
2025-04-01
DOI
https://doi.org/10.1063/5.0261501
Citations
1
Primary Topic
Ga2O3 and related materials
Type
article
Field-Weighted Citation Impact
0.43

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article

β-Ga2O3:Cr nanowires with optical microcavities for determining local heating induced by x-ray nanobeams

Jaime Dolado, Gema Martínez‐Criado, M.L. Nó, Beatriz Rodríguez et al.
1 citations
APL Materials
Ga2O3 and related materials
0.43
article

β-Ga2O3:Cr nanowires with optical microcavities for determining local heating induced by x-ray nanobeams

Jaime Dolado, Gema Martínez‐Criado, M.L. Nó, Beatriz Rodríguez, Bianchi Méndez, Pedro Hidalgo, Emilio Nogales, J. San Juán, Manuel Alonso‐Orts, Daniel Carrasco, Paula Pérez‐Peinado
article en
1 citations

Abstract

This study explores the x-ray excited optical luminescence (XEOL) of optical microcavities fabricated in β-Ga2O3:Cr nanowires (NWs). XEOL measurements reveal prominent luminescence bands in the near ultraviolet-blue (NUV-B) and in the red-near infrared (R-NIR) spectral regions. The NUV-B emission originates from β-Ga2O3 defects, while the R-NIR band is attributed to Cr3+ intraionic transitions. Both spectral regions exhibit sharp resonances, which are analyzed as Fabry–Pérot and whispering gallery mode resonances. Exposure to x-ray nanobeam induces a redshift of the sharp R-NIR peaks, attributed to local temperature increase in the NWs caused by x-ray absorption. The influence of this temperature rise on the NUV-B peaks is also evaluated. In addition, the local temperature increase due to x-ray absorption is estimated through COMSOL finite-difference time-domain simulations, incorporating the material’s physical and thermal properties. This work demonstrates the application of β-Ga2O3:Cr optical microcavities as luminescence-based nanothermometers to probe the localized effects of x-ray nanobeam irradiation.

APL MaterialsVol. 13(4)
Universidad Complutense de Madrid (ES), University of the Basque Country (ES), University of Bremen (DE), European Synchrotron Radiation Facility (FR), Instituto de Ciencia de Materiales de Madrid (ES)
Comunidad de Madrid, Deutsche Forschungsgemeinschaft, European Synchrotron Radiation Facility, Ministerio de Ciencia e Innovación, Universität Bremen, Air Force Office of Scientific Research
Openalex Percentile: Top 43%
Ga2O3 and related materials
0.43
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