Tunable Ultrastrong Magnon–Magnon Coupling Approaching the Deep-Strong Regime in a van der Waals Antiferromagnet
Antiferromagnetic (AFM) magnons in van der Waals (vdW) materials offer substantial potential for applications in magnonics and spintronics. In this study, we demonstrate ultrastrong magnon-magnon coupling in the GHz regime within a vdW AFM, achieving a maximum coupling rate of 0.91. Our investigation shows the tunability of coupling strength through temperature-dependent magnetic anisotropies. We compare coupling strength values derived from the gap size from the measured spectrum with those calculated directly through the coupling parameter and show that the gap size as a measure of coupling strength is limited for the ultrastrong coupling regime. Additionally, analytical calculations show the possibility to reach the deep-strong coupling regime by engineering the magnetic anisotropy. These findings highlight the potential of vdW AFMs as a model case to study magnetization dynamics in low-symmetry magnetic materials.
Authors
- C. W. F. Freeman
- Adam K. Budniak (ORCID: https://orcid.org/0000-0001-7073-8279)
- Michel Bosman (ORCID: https://orcid.org/0000-0002-8717-7655)
- Goki Eda (ORCID: https://orcid.org/0000-0002-1575-8020)
- Thomas Thomson (ORCID: https://orcid.org/0000-0002-4110-1567)
- H. Kurebayashi (ORCID: https://orcid.org/0000-0002-2021-1556)
- Henry De Libero
- Harry Youel (ORCID: https://orcid.org/0009-0007-3004-6367)
- M. Cubukcu (ORCID: https://orcid.org/0000-0003-4086-0067)
- Zekun Xue
Institutions
- Agency for Science, Technology and Research (SG)
- National Physical Laboratory (GB)
- National University of Singapore (SG)
- Tohoku University (JP)
- London Centre for Nanotechnology (GB)
- University of Manchester (GB)
- Centre of Excellence for Advanced Materials (CN)
- Institute for Materials Research, Tohoku University
- University College London (GB)
Publication Details
- Journal
- ACS Nano
- Published
- 2025-04-17
- DOI
- https://doi.org/10.1021/acsnano.5c02576
- Citations
- 6
- Primary Topic
- Topological Materials and Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 7.48
Funders
- UK Research and Innovation
- Ministry of Education - Singapore
- Engineering and Physical Sciences Research Council