Scaling law and extrinsic mechanisms for time-reversal-odd second-order nonlinear transport

Time-reversal-odd ($\mathcal{T}$-odd) second-order nonlinear current response has been theoretically proposed and experimentally confirmed recently. However, the role of disorder scattering in the response, especially whether it contributes to the ${\ensuremath{\sigma}}_{xx}$-independent term, has not been clarified. Here, we derive a general scaling law for this effect, which accounts for multiple scattering sources. We show that the nonlinear conductivity is generally a quartic function in ${\ensuremath{\sigma}}_{xx}$. The microscopic mechanisms underlying each scaling term are revealed, which include multiple previously unknown extrinsic processes unique to $\mathcal{T}$-odd nonlinear transport. Besides intrinsic contribution, we find that extrinsic contributions also enter the zeroth-order term, and their values can be comparable to or even larger than the intrinsic one. This offers a solution to the conflicting interpretations of recent experiments. In addition, cubic and quartic terms must involve skew scattering, and they signal competition between at least two scattering sources. Our finding reveals the significant role of disorder scattering in $\mathcal{T}$-odd nonlinear transport, and it establishes a foundation for analyzing experimental results.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-04-16
DOI
https://doi.org/10.1103/physrevb.111.155127
Citations
16
Primary Topic
Random lasers and scattering media
Type
article
Field-Weighted Citation Impact
20.81

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article

Scaling law and extrinsic mechanisms for time-reversal-odd second-order nonlinear transport

Shengyuan A. Yang, Cong Xiao, Yue-Xin Huang, Xiao Li
16 citations
Physical review. B./Physical review. B
Random lasers and scattering media
20.81
article

Scaling law and extrinsic mechanisms for time-reversal-odd second-order nonlinear transport

Shengyuan A. Yang, Cong Xiao, Yue-Xin Huang, Xiao Li
article en
16 citations

Abstract

Time-reversal-odd ($\mathcal{T}$-odd) second-order nonlinear current response has been theoretically proposed and experimentally confirmed recently. However, the role of disorder scattering in the response, especially whether it contributes to the ${\ensuremath{\sigma}}_{xx}$-independent term, has not been clarified. Here, we derive a general scaling law for this effect, which accounts for multiple scattering sources. We show that the nonlinear conductivity is generally a quartic function in ${\ensuremath{\sigma}}_{xx}$. The microscopic mechanisms underlying each scaling term are revealed, which include multiple previously unknown extrinsic processes unique to $\mathcal{T}$-odd nonlinear transport. Besides intrinsic contribution, we find that extrinsic contributions also enter the zeroth-order term, and their values can be comparable to or even larger than the intrinsic one. This offers a solution to the conflicting interpretations of recent experiments. In addition, cubic and quartic terms must involve skew scattering, and they signal competition between at least two scattering sources. Our finding reveals the significant role of disorder scattering in $\mathcal{T}$-odd nonlinear transport, and it establishes a foundation for analyzing experimental results.

Physical review. B./Physical review. BVol. 111(15)
City University of Hong Kong (HK), University of Macau (MO), Fudan University (CN), Bay Institute (US), Great Bay University
City University of Hong Kong, National Natural Science Foundation of China, Science and Technology Development Fund
Openalex Percentile: Top 0%
Random lasers and scattering media
20.81
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Scaling law and extrinsic mechanisms for time-reversal-odd second-order nonlinear transport — Shengyuan A. Yang, Cong Xiao, et al. · Physical review. B./Physical review. B (2025) | TGRS Research Map | TGRS