Resonant propagation of extreme-ultraviolet pulses through strongly driven high-density media

We show that by combining strong-field dressing and resonant propagation of XUV pulses, the transition of absorption lines from their natural Lorentzian profiles through Fano and complex multipeak shapes all the way back to broadened near-Lorentzian profiles can be achieved, in the limit of optically thick samples. The final stage of this spectral modification can be understood in terms of a significant temporal stretching and delay of the resonant XUV pulse as it propagates through the dense gas, which alters the ultrafast absorption that is modified by the time-synchronized few-femtosecond laser pulse. We first demonstrate this concept in numerical calculations, both using a model system and through a fully coupled solution of the time-dependent Schrödinger equation and the Maxwell wave equation. The applicability and generality of the underlying mechanism is then illustrated in proof-of-principle attosecond transient absorption measurements in a helium gas with a widely varying atomic density. These results provide insights into the interaction of ultrashort laser pulses with dense media and its coherent control.

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Publication Details

Journal
Physical Review Research
Published
2025-04-16
DOI
https://doi.org/10.1103/physrevresearch.7.023064
Citations
1
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
1.25

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article

Resonant propagation of extreme-ultraviolet pulses through strongly driven high-density media

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Laser-Matter Interactions and Applications
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article

Resonant propagation of extreme-ultraviolet pulses through strongly driven high-density media

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article en
1 citations

Abstract

We show that by combining strong-field dressing and resonant propagation of XUV pulses, the transition of absorption lines from their natural Lorentzian profiles through Fano and complex multipeak shapes all the way back to broadened near-Lorentzian profiles can be achieved, in the limit of optically thick samples. The final stage of this spectral modification can be understood in terms of a significant temporal stretching and delay of the resonant XUV pulse as it propagates through the dense gas, which alters the ultrafast absorption that is modified by the time-synchronized few-femtosecond laser pulse. We first demonstrate this concept in numerical calculations, both using a model system and through a fully coupled solution of the time-dependent Schrödinger equation and the Maxwell wave equation. The applicability and generality of the underlying mechanism is then illustrated in proof-of-principle attosecond transient absorption measurements in a helium gas with a widely varying atomic density. These results provide insights into the interaction of ultrashort laser pulses with dense media and its coherent control.

Physical Review ResearchVol. 7(2)
Louisiana State University (US), Tianjin University (CN), Max Planck Institute for Nuclear Physics (DE), Lanzhou University (CN)
U.S. Department of Energy, National Natural Science Foundation of China, Office of Science, Basic Energy Sciences
Openalex Percentile: Top 22%
Laser-Matter Interactions and Applications
1.25
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