A Circular Photogalvanic Effect-Controlled Polarimeter based on a Bipolar Phototransistor Utilized in Spatially Resolved Mapping

The circular photogalvanic effect (CPGE), converted from the photon angular moment as a spin-polarized charge current via inversion asymmetry, is an effective approach to detecting circularly polarized light. However, the CPGE current is typically weak, and even the electrical gate gives quite limited improvement, necessitating the use of auxiliary amplifiers to strengthen the signals for practical applications. Here, we constitute a vertical bipolar phototransistor based on MoS<sub>2</sub>/ZrGeTe<sub>4</sub>/MoS<sub>2</sub> heterojunction with a noncentrosymmetric active region, which can detect and amplify the CPGE photocurrents for all directions, with a CPGE gain of 25. Thereupon, we achieve tens of μA/W CPGE responsivity from visible to near-infrared (NIR) and wide acceptance angles from 45° to -45° at room temperature, revealing multiscenario applications. The full Stokes spatially resolved mapping of the NIR vortex beam demonstrates its practical applicability as a polarimeter with high sensitivity. Our work provides an approach to developing nanostructured polarimeters controlled by inversion symmetry and devoid of external amplification modules, which leads to potential applications for future nanophotonics and optoelectronic nanodevices.

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Publication Details

Journal
ACS Nano
Published
2025-04-16
DOI
https://doi.org/10.1021/acsnano.4c18833
Citations
1
Primary Topic
Optical Polarization and Ellipsometry
Type
article
Field-Weighted Citation Impact
0.67

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article

A Circular Photogalvanic Effect-Controlled Polarimeter based on a Bipolar Phototransistor Utilized in Spatially Resolved Mapping

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1 citations
ACS Nano
Optical Polarization and Ellipsometry
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article

A Circular Photogalvanic Effect-Controlled Polarimeter based on a Bipolar Phototransistor Utilized in Spatially Resolved Mapping

Weibo Gao, Ruixue Bai, Yaojie Zhu, Rui Zhou, Xilin Zhang, Zuowei Yan, Xiaoshan Du, Hui Ma, Yulun Liu
article en
1 citations

Abstract

The circular photogalvanic effect (CPGE), converted from the photon angular moment as a spin-polarized charge current via inversion asymmetry, is an effective approach to detecting circularly polarized light. However, the CPGE current is typically weak, and even the electrical gate gives quite limited improvement, necessitating the use of auxiliary amplifiers to strengthen the signals for practical applications. Here, we constitute a vertical bipolar phototransistor based on MoS<sub>2</sub>/ZrGeTe<sub>4</sub>/MoS<sub>2</sub> heterojunction with a noncentrosymmetric active region, which can detect and amplify the CPGE photocurrents for all directions, with a CPGE gain of 25. Thereupon, we achieve tens of μA/W CPGE responsivity from visible to near-infrared (NIR) and wide acceptance angles from 45° to -45° at room temperature, revealing multiscenario applications. The full Stokes spatially resolved mapping of the NIR vortex beam demonstrates its practical applicability as a polarimeter with high sensitivity. Our work provides an approach to developing nanostructured polarimeters controlled by inversion symmetry and devoid of external amplification modules, which leads to potential applications for future nanophotonics and optoelectronic nanodevices.

ACS NanoVol. 19(16)
Centre for Quantum Technologies (SG), National University of Singapore (SG), Nanyang Technological University (SG), Tiangong University (CN), Nankai University (CN), Photonic Science (United Kingdom) (GB), Optica (US)
National Natural Science Foundation of China, Nankai University, Natural Science Foundation of Tianjin City, Tianjin Municipal Education Commission, Key Technologies Research and Development Program
Affordable and clean energy
Openalex Percentile: Top 33%
Optical Polarization and Ellipsometry
0.67
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