The effects of disorder in superconducting materials on qubit coherence

Introducing disorder in the superconducting materials has been considered promising to enhance the electromagnetic impedance and realize noise-resilient superconducting qubits. Despite a number of pioneering implementations, the understanding of the correlation between the material disorder and the qubit coherence is still developing. Here, we demonstrate a systematic characterization of fluxonium qubits with the superinductors made by spinodal titanium-aluminum-nitride with varied disorder. From qubit noise spectroscopy, the flux noise and the dielectric loss are extracted as a measure of the coherence properties. Our results reveal that the 1/f <sup>α</sup> flux noise dominates the qubit decoherence around the flux-frustration point, strongly correlated with the material disorder; while the dielectric loss are largely similar under a wide range of material properties. From the flux-noise amplitudes, the areal density (σ) of the phenomenological spin defects and material disorder are found to be approximately correlated by <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>σ</mml:mi> <mml:mo>∝</mml:mo> <mml:msubsup><mml:mrow><mml:mi>ρ</mml:mi></mml:mrow> <mml:mrow><mml:mi>x</mml:mi> <mml:mi>x</mml:mi></mml:mrow> <mml:mrow><mml:mn>3</mml:mn></mml:mrow> </mml:msubsup> </mml:math> , or effectively <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msup> <mml:mrow><mml:mrow><mml:mo>(</mml:mo> <mml:mrow> <mml:msub><mml:mrow><mml:mi>k</mml:mi></mml:mrow> <mml:mrow><mml:mi>F</mml:mi></mml:mrow> </mml:msub> <mml:mi>l</mml:mi></mml:mrow> <mml:mo>)</mml:mo></mml:mrow> </mml:mrow> <mml:mrow><mml:mo>-</mml:mo> <mml:mn>3</mml:mn></mml:mrow> </mml:msup> </mml:math> . This work has provided new insights on the origin of decoherence channels beyond surface defects and within the superconductors, and could serve as a useful guideline for material design and optimization.

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Publication Details

Journal
Nature Communications
Published
2025-04-16
DOI
https://doi.org/10.1038/s41467-025-58745-y
Citations
2
Primary Topic
Quantum and electron transport phenomena
Type
article
Field-Weighted Citation Impact
2.49

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article

The effects of disorder in superconducting materials on qubit coherence

Hui‐Hai Zhao, Xiaohe Miao, Hantao Sun, Hao Deng et al.
2 citations
Nature Communications
Quantum and electron transport phenomena
2.49
article

The effects of disorder in superconducting materials on qubit coherence

Hui‐Hai Zhao, Xiaohe Miao, Hantao Sun, Hao Deng, Tian Xia, Xizheng Ma, Feng Wu, Chao Zhang, Jianjun Chen, Fei Wang, Zhijun Song, Make Ying, Ran Gao, Xin Wan, Yaoyun Shi, Chunqing Deng
article en
2 citations

Abstract

Introducing disorder in the superconducting materials has been considered promising to enhance the electromagnetic impedance and realize noise-resilient superconducting qubits. Despite a number of pioneering implementations, the understanding of the correlation between the material disorder and the qubit coherence is still developing. Here, we demonstrate a systematic characterization of fluxonium qubits with the superinductors made by spinodal titanium-aluminum-nitride with varied disorder. From qubit noise spectroscopy, the flux noise and the dielectric loss are extracted as a measure of the coherence properties. Our results reveal that the 1/f <sup>α</sup> flux noise dominates the qubit decoherence around the flux-frustration point, strongly correlated with the material disorder; while the dielectric loss are largely similar under a wide range of material properties. From the flux-noise amplitudes, the areal density (σ) of the phenomenological spin defects and material disorder are found to be approximately correlated by <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:mi>σ</mml:mi> <mml:mo>∝</mml:mo> <mml:msubsup><mml:mrow><mml:mi>ρ</mml:mi></mml:mrow> <mml:mrow><mml:mi>x</mml:mi> <mml:mi>x</mml:mi></mml:mrow> <mml:mrow><mml:mn>3</mml:mn></mml:mrow> </mml:msubsup> </mml:math> , or effectively <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"> <mml:msup> <mml:mrow><mml:mrow><mml:mo>(</mml:mo> <mml:mrow> <mml:msub><mml:mrow><mml:mi>k</mml:mi></mml:mrow> <mml:mrow><mml:mi>F</mml:mi></mml:mrow> </mml:msub> <mml:mi>l</mml:mi></mml:mrow> <mml:mo>)</mml:mo></mml:mrow> </mml:mrow> <mml:mrow><mml:mo>-</mml:mo> <mml:mn>3</mml:mn></mml:mrow> </mml:msup> </mml:math> . This work has provided new insights on the origin of decoherence channels beyond surface defects and within the superconductors, and could serve as a useful guideline for material design and optimization.

Nature CommunicationsVol. 16(1)
Peking University (CN), Westlake University (CN), National Institutes for Quantum Science and Technology (JP), Zhejiang Lab (CN), Hangzhou Vocational and Technical College (CN), QuantumCTek (China) (CN), Quantum Design (United States) (US), Jordan Valley Semiconductors (China) (CN), Quantum Technologies (Sweden) (SE), Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area (CN), United Microelectronics (United States) (US)
Westlake University
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Openalex Percentile: Top 12%
Quantum and electron transport phenomena
2.49
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