Pressure-induced redistribution in density of states and reemergence of superconductivity in AgSnSe2

The intricate relationship between superconductivity and disorder is a captivating subject within condensed matter physics. Strong disorder suppresses superconductivity and induces a superconductor-insulator transition. However, below a certain critical degree of disorder, the superconductivity critical temperature (<i>T</i> <sub>c</sub>) can be enhanced. Herein, we present evidence of pressure-induced reemergence of superconductivity in a strongly disordered 3D superconductor AgSnSe<sub>2</sub>. A structural phase transition from NaCl- to CsCl-type structure occurs, coinciding with the emergence of the second superconducting state. First-principles calculations suggest that the partial density of states in Se atoms exhibits a sharp elevation around the transition pressure, which is related to the secondary superconducting state. Our study illustrates AgSnSe<sub>2</sub> as a promising platform to explore the comprehensive effects among disorder, high pressure, and superconductivity, offering insights for subsequent experimental and theoretical studies.

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Publication Details

Journal
iScience
Published
2025-04-15
DOI
https://doi.org/10.1016/j.isci.2025.112442
Primary Topic
Chalcogenide Semiconductor Thin Films
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article
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article

Pressure-induced redistribution in density of states and reemergence of superconductivity in AgSnSe2

Tianping Ying, Cuiying Pei, Junjie Wang, Yuyang Jiang et al.
iScience
Chalcogenide Semiconductor Thin Films
article

Pressure-induced redistribution in density of states and reemergence of superconductivity in AgSnSe2

Tianping Ying, Cuiying Pei, Junjie Wang, Yuyang Jiang, Juefei Wu, Weizheng Cao, Yanpeng Qi, Qi Wang, Yi Zhao
article en

Abstract

The intricate relationship between superconductivity and disorder is a captivating subject within condensed matter physics. Strong disorder suppresses superconductivity and induces a superconductor-insulator transition. However, below a certain critical degree of disorder, the superconductivity critical temperature (<i>T</i> <sub>c</sub>) can be enhanced. Herein, we present evidence of pressure-induced reemergence of superconductivity in a strongly disordered 3D superconductor AgSnSe<sub>2</sub>. A structural phase transition from NaCl- to CsCl-type structure occurs, coinciding with the emergence of the second superconducting state. First-principles calculations suggest that the partial density of states in Se atoms exhibits a sharp elevation around the transition pressure, which is related to the secondary superconducting state. Our study illustrates AgSnSe<sub>2</sub> as a promising platform to explore the comprehensive effects among disorder, high pressure, and superconductivity, offering insights for subsequent experimental and theoretical studies.

iScienceVol. 28(5)
Chinese Academy of Sciences (CN), ShanghaiTech University (CN), Institute of Physics (CN)
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Chalcogenide Semiconductor Thin Films
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