Infrared Metaplasmonics

Plasmonic response in metals, defined as the ability to support subwavelength confinement of surface plasmon modes, is typically limited to a narrow frequency range below the metals’ plasma frequency. This places severe limitations on the operational wavelengths of plasmonic materials and devices. However, when the volume of a metal film is massively decreased, highly confined quasi-two-dimensional surface plasmon modes can be supported out to wavelengths well beyond the plasma wavelength. While this has, thus far, been achieved using ultrathin (nm-scale) metals, such films are quite difficult to realize and suffer from even higher losses than bulk plasmonic films. To extend the plasmonic response to the infrared, here we introduce the concept of metaplasmonics, representing a novel plasmonic modality with a host of appealing properties. By fabricating and characterizing a series of metaplasmonic nanoribbons, we demonstrate large confinement, high-quality factors, and large near-field enhancements across a broad wavelength range, extending well beyond the limited bandwidth of traditional plasmonic materials. We demonstrate 35× plasmon wavelength reduction, and numerical simulations suggest that further wavelength reduction, up to a factor of 150, is achievable using our approach. The demonstration of the metaplasmonics paradigm offers a promising path to fill the near- and mid-infrared technological gap for high-quality plasmonic materials and provides a new material system to study the effects of extreme plasmonic confinement for applications in nonlinear and quantum plasmonics.

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Publication Details

Journal
ACS Photonics
Published
2025-04-15
DOI
https://doi.org/10.1021/acsphotonics.5c00147
Citations
3
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
2.02

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article

Infrared Metaplasmonics

Alexander Ware, Zarko Sakotic, Daniel Wasserman, Divya Hungund et al.
3 citations
ACS Photonics
Plasmonic and Surface Plasmon Research
2.02
article

Infrared Metaplasmonics

Alexander Ware, Zarko Sakotic, Daniel Wasserman, Divya Hungund, Amogh Raju, Noah Mansfeld, Daniel Krueger
article en
3 citations

Abstract

Plasmonic response in metals, defined as the ability to support subwavelength confinement of surface plasmon modes, is typically limited to a narrow frequency range below the metals’ plasma frequency. This places severe limitations on the operational wavelengths of plasmonic materials and devices. However, when the volume of a metal film is massively decreased, highly confined quasi-two-dimensional surface plasmon modes can be supported out to wavelengths well beyond the plasma wavelength. While this has, thus far, been achieved using ultrathin (nm-scale) metals, such films are quite difficult to realize and suffer from even higher losses than bulk plasmonic films. To extend the plasmonic response to the infrared, here we introduce the concept of metaplasmonics, representing a novel plasmonic modality with a host of appealing properties. By fabricating and characterizing a series of metaplasmonic nanoribbons, we demonstrate large confinement, high-quality factors, and large near-field enhancements across a broad wavelength range, extending well beyond the limited bandwidth of traditional plasmonic materials. We demonstrate 35× plasmon wavelength reduction, and numerical simulations suggest that further wavelength reduction, up to a factor of 150, is achievable using our approach. The demonstration of the metaplasmonics paradigm offers a promising path to fill the near- and mid-infrared technological gap for high-quality plasmonic materials and provides a new material system to study the effects of extreme plasmonic confinement for applications in nonlinear and quantum plasmonics.

ACS PhotonicsVol. 12(5)
The University of Texas at Austin (US)
Defense Advanced Research Projects Agency, Division of Materials Research
Openalex Percentile: Top 15%
Plasmonic and Surface Plasmon Research
2.02
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