Evidence for reduced periodic lattice distortion within the Sb-terminated surface layer of the kagome metal <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi>CsV</mml:mi></mml:mrow><mml:mn>3</mml:mn></mml:msub><mml:

The discovery of the kagome metal <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:msub><a:mrow><a:mi>CsV</a:mi></a:mrow><a:mn>3</a:mn></a:msub><a:msub><a:mrow><a:mi>Sb</a:mi></a:mrow><a:mn>5</a:mn></a:msub></a:math> sparked broad interest, due to the coexistence of a charge density wave (CDW) phase and possible unconventional superconductivity in the material. In this Letter, we use low-energy electron diffraction (LEED) with a <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mi>µ</b:mi><b:mi mathvariant="normal">m</b:mi></b:math>-sized electron beam to explore the periodic lattice distortion at the antimony-terminated surface in the CDW phase. We recorded high-quality backscattering diffraction patterns in ultrahigh vacuum from multiple cleaved samples. Unexpectedly, we did not find superstructure reflexes at intensity levels predicted from dynamical LEED calculations for the reported <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"><d:mrow><d:mn>2</d:mn><d:mo>×</d:mo><d:mn>2</d:mn><d:mo>×</d:mo><d:mn>2</d:mn></d:mrow></d:math> bulk structure. Our results suggest that in <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"><e:msub><e:mrow><e:mi>CsV</e:mi></e:mrow><e:mn>3</e:mn></e:msub><e:msub><e:mrow><e:mi>Sb</e:mi></e:mrow><e:mn>5</e:mn></e:msub></e:math> the periodic lattice distortion accompanying the CDW is less pronounced at Sb-terminated surfaces than in the bulk.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-04-09
DOI
https://doi.org/10.1103/physrevb.111.l140101
Citations
3
Primary Topic
Topological Materials and Phenomena
Type
article
Field-Weighted Citation Impact
3.74

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article

Evidence for reduced periodic lattice distortion within the Sb-terminated surface layer of the kagome metal <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi>CsV</mml:mi></mml:mrow><mml:mn>3</mml:mn></mml:msub><mml:

I. Vinograd, Claus Ropers, Felix Kurtz, Amir A. Haghighirad et al.
3 citations
Physical review. B./Physical review. B
Topological Materials and Phenomena
3.74
article

Evidence for reduced periodic lattice distortion within the Sb-terminated surface layer of the kagome metal <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mrow><mml:mi>CsV</mml:mi></mml:mrow><mml:mn>3</mml:mn></mml:msub><mml:

I. Vinograd, Claus Ropers, Felix Kurtz, Amir A. Haghighirad, Chandra Shekhar, Alp Akbıyık, M. Le Tacon, Gevin von Witte, Claudia Felser, Dong Chen, Lukas Jehn
article en
3 citations

Abstract

The discovery of the kagome metal <a:math xmlns:a="http://www.w3.org/1998/Math/MathML"><a:msub><a:mrow><a:mi>CsV</a:mi></a:mrow><a:mn>3</a:mn></a:msub><a:msub><a:mrow><a:mi>Sb</a:mi></a:mrow><a:mn>5</a:mn></a:msub></a:math> sparked broad interest, due to the coexistence of a charge density wave (CDW) phase and possible unconventional superconductivity in the material. In this Letter, we use low-energy electron diffraction (LEED) with a <b:math xmlns:b="http://www.w3.org/1998/Math/MathML"><b:mi>µ</b:mi><b:mi mathvariant="normal">m</b:mi></b:math>-sized electron beam to explore the periodic lattice distortion at the antimony-terminated surface in the CDW phase. We recorded high-quality backscattering diffraction patterns in ultrahigh vacuum from multiple cleaved samples. Unexpectedly, we did not find superstructure reflexes at intensity levels predicted from dynamical LEED calculations for the reported <d:math xmlns:d="http://www.w3.org/1998/Math/MathML"><d:mrow><d:mn>2</d:mn><d:mo>×</d:mo><d:mn>2</d:mn><d:mo>×</d:mo><d:mn>2</d:mn></d:mrow></d:math> bulk structure. Our results suggest that in <e:math xmlns:e="http://www.w3.org/1998/Math/MathML"><e:msub><e:mrow><e:mi>CsV</e:mi></e:mrow><e:mn>3</e:mn></e:msub><e:msub><e:mrow><e:mi>Sb</e:mi></e:mrow><e:mn>5</e:mn></e:msub></e:math> the periodic lattice distortion accompanying the CDW is less pronounced at Sb-terminated surfaces than in the bulk.

Physical review. B./Physical review. BVol. 111(14)
Karlsruhe Institute of Technology (DE), ETH Zurich (CH), Institute for Biomedical Engineering (CH), Max Planck Institute for Chemical Physics of Solids (DE), Max Planck Institute for Multidisciplinary Sciences (DE), University of Göttingen (DE)
Deutsche Forschungsgemeinschaft, Max Planck School of Photonics, European Research Council
Openalex Percentile: Top 8%
Topological Materials and Phenomena
3.74
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