Light-Field Dressing of Transient Photoexcited States above the Fermi Energy
Time-periodic light field provides an emerging pathway for dynamically engineering quantum materials by forming hybrid states between photons and Bloch electrons. So far, experimental progress on light-field dressed states has been mainly focused on the occupied states; however, it is unclear if the transient photoexcited states above the Fermi energy E_{F} can also be dressed, leaving the dynamical interplay between photoexcitation and light-field dressing elusive. Here, we provide direct experimental evidence for light-field dressing of the transient photoexcited surface states above E_{F}, which exhibits distinct dynamics with a delay response as compared to light-field dressed states below E_{F}. Our work reveals the dual roles of the pump pulse in both photoexcitation and light-field dressing, providing a more comprehensive picture with new insights on the light-induced manipulation of transient electronic states.
Authors
- Shuyun Zhou (ORCID: https://orcid.org/0000-0002-9841-8610)
- Wanying Chen (ORCID: https://orcid.org/0000-0002-8650-4888)
- Tianyun Lin (ORCID: https://orcid.org/0000-0002-4541-7171)
- Fei Wang (ORCID: https://orcid.org/0009-0009-4585-1726)
- Haoyuan Zhong (ORCID: https://orcid.org/0000-0003-0453-3405)
- Changhua Bao (ORCID: https://orcid.org/0000-0002-8706-6541)
- Hong‐Yun Zhang (ORCID: https://orcid.org/0000-0002-0993-8949)
Institutions
- Tsinghua University (CN)
Publication Details
- Journal
- Physical Review Letters
- Published
- 2025-04-07
- DOI
- https://doi.org/10.1103/physrevlett.134.146401
- Citations
- 1
- Primary Topic
- Topological Materials and Phenomena
- Type
- article
- Field-Weighted Citation Impact
- 1.25
Funders
- National Natural Science Foundation of China
- National Key Research and Development Program of China