Coherent superposition mediating energy flow between fundamental and third-harmonic modes

We predict a coherent superposition mediating a significant periodic energy flow between the fundamental and third-harmonic modes. It is found for the linearly polarized electromagnetic field, where a lower bound $S$ state $|g\ensuremath{\rangle}$ is coupled to an upper bound $S$ state $|b\ensuremath{\rangle}$, where the energy difference between these states is about two photons and the coupling occurs due to the above threshold ionization from these states together. Exceptional point on complex quasienergy surfaces of the dressed resonances $|g\ensuremath{\rangle}$ and $|b\ensuremath{\rangle}$ indicates coherent superposition that manifests itself dynamically as the Rabi cycle. The cycle is irreversible, being gradually quenched by the above threshold ionization while emitting strong third-harmonic and fundamental pulses. We provide a numerical evidence confirming the existence of such a process in the helium atom.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-04-04
DOI
https://doi.org/10.1103/physreva.111.043105
Primary Topic
Laser-Matter Interactions and Applications
Type
article
Field-Weighted Citation Impact
0.00

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article

Coherent superposition mediating energy flow between fundamental and third-harmonic modes

Petra Ruth Kaprálová-Žďánská
Physical review. A/Physical review, A
Laser-Matter Interactions and Applications
article

Coherent superposition mediating energy flow between fundamental and third-harmonic modes

Petra Ruth Kaprálová-Žďánská
article en

Abstract

We predict a coherent superposition mediating a significant periodic energy flow between the fundamental and third-harmonic modes. It is found for the linearly polarized electromagnetic field, where a lower bound $S$ state $|g\ensuremath{\rangle}$ is coupled to an upper bound $S$ state $|b\ensuremath{\rangle}$, where the energy difference between these states is about two photons and the coupling occurs due to the above threshold ionization from these states together. Exceptional point on complex quasienergy surfaces of the dressed resonances $|g\ensuremath{\rangle}$ and $|b\ensuremath{\rangle}$ indicates coherent superposition that manifests itself dynamically as the Rabi cycle. The cycle is irreversible, being gradually quenched by the above threshold ionization while emitting strong third-harmonic and fundamental pulses. We provide a numerical evidence confirming the existence of such a process in the helium atom.

Physical review. A/Physical review, AVol. 111(4)
Czech Academy of Sciences (CZ), FZU ‒ Institute of Physics of the Academy of Sciences of the Czech Republic (CZ)
Universität Heidelberg, Grantová Agentura České Republiky
Affordable and clean energy
Openalex Percentile: Top 95%
Laser-Matter Interactions and Applications
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