Multi‐Model Assessment of Future Hydrogen Soil Deposition and Lifetime Using CMIP6 Data

Abstract Atmospheric hydrogen indirectly contributes to greenhouse warming by extending methane lifetime, and increasing stratospheric water vapor and tropospheric ozone. Its main sinks are oxidation with OH, and dry deposition via microbial soil uptake. The latter accounts for approximately of the sink and is poorly constrained under present day conditions, with very limited studies on its future evolution. This work uses an offline hydrogen deposition scheme to perform the first multi‐model assessment of deposition velocities driven using data from five models from the Coupled Model Intercomparison Phase 6 project. Deposition values calculated from historical data are compared to observations, and deposition velocities are evaluated across four scenarios . We find deposition velocity increases with time and stronger climate forcing. A 20 present‐day, inter‐model discrepancy, linked to differences in soil moisture and porosity, leads to a 33 variation in hydrogen's global warming potential over a 100‐year time horizon.

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Publication Details

Journal
Geophysical Research Letters
Published
2025-04-01
DOI
https://doi.org/10.1029/2024gl113653
Citations
7
Primary Topic
Atmospheric and Environmental Gas Dynamics
Type
article
Field-Weighted Citation Impact
7.74
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article

Multi‐Model Assessment of Future Hydrogen Soil Deposition and Lifetime Using CMIP6 Data

Alexander T. Archibald, N. J. Warwick, Megan Brown
7 citations
Geophysical Research Letters
Atmospheric and Environmental Gas Dynamics
7.74
article

Multi‐Model Assessment of Future Hydrogen Soil Deposition and Lifetime Using CMIP6 Data

Alexander T. Archibald, N. J. Warwick, Megan Brown
article en
7 citations

Abstract

Abstract Atmospheric hydrogen indirectly contributes to greenhouse warming by extending methane lifetime, and increasing stratospheric water vapor and tropospheric ozone. Its main sinks are oxidation with OH, and dry deposition via microbial soil uptake. The latter accounts for approximately of the sink and is poorly constrained under present day conditions, with very limited studies on its future evolution. This work uses an offline hydrogen deposition scheme to perform the first multi‐model assessment of deposition velocities driven using data from five models from the Coupled Model Intercomparison Phase 6 project. Deposition values calculated from historical data are compared to observations, and deposition velocities are evaluated across four scenarios . We find deposition velocity increases with time and stronger climate forcing. A 20 present‐day, inter‐model discrepancy, linked to differences in soil moisture and porosity, leads to a 33 variation in hydrogen's global warming potential over a 100‐year time horizon.

Geophysical Research LettersVol. 52(7)
University of Cambridge (GB), National Centre for Atmospheric Science (GB)
Openalex Percentile: Top 3%
Atmospheric and Environmental Gas Dynamics
7.74
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