Continuum model of strong light-matter coupling for molecular polaritons

Strong coupling between light and matter generates hybrid polariton modes. We present a continuum formalism that expresses the polariton modes in terms of light and matter densities of states (DOS). We derive exact expressions for the light and matter DOS for a planar cavity containing a strongly dispersive dielectric. We show that these DOS depend exclusively on the linear response of the cavity components, i.e., the reflectance of the mirrors and the susceptibility of the dielectric. We further show that, within the strong coupling regime, the light and matter DOS are well approximated by coupled mode theory. Altogether, our continuum formalism offers a unified treatment of polaritons that connects the framework of light-matter coupling with that of linear dispersion.

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Publication Details

Journal
Physical review. B./Physical review. B
Published
2025-03-31
DOI
https://doi.org/10.1103/physrevb.111.104209
Citations
3
Primary Topic
Strong Light-Matter Interactions
Type
article
Field-Weighted Citation Impact
3.74

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article

Continuum model of strong light-matter coupling for molecular polaritons

Suman Gunasekaran, Andrew J. Musser, Ryan F. Pinard
3 citations
Physical review. B./Physical review. B
Strong Light-Matter Interactions
3.74
article

Continuum model of strong light-matter coupling for molecular polaritons

Suman Gunasekaran, Andrew J. Musser, Ryan F. Pinard
article en
3 citations

Abstract

Strong coupling between light and matter generates hybrid polariton modes. We present a continuum formalism that expresses the polariton modes in terms of light and matter densities of states (DOS). We derive exact expressions for the light and matter DOS for a planar cavity containing a strongly dispersive dielectric. We show that these DOS depend exclusively on the linear response of the cavity components, i.e., the reflectance of the mirrors and the susceptibility of the dielectric. We further show that, within the strong coupling regime, the light and matter DOS are well approximated by coupled mode theory. Altogether, our continuum formalism offers a unified treatment of polaritons that connects the framework of light-matter coupling with that of linear dispersion.

Physical review. B./Physical review. BVol. 111(10)
Cornell University (US)
U.S. Department of Energy, Alfred P. Sloan Foundation, Arnold and Mabel Beckman Foundation, Cornell University, Office of Science, Basic Energy Sciences
Climate action
Openalex Percentile: Top 8%
Strong Light-Matter Interactions
3.74
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