Modeling the Black and Brown Carbon Absorption and Their Radiative Impact: The June 2023 Intense Canadian Boreal Wildfires Case Study

Abstract Black carbon (BC) and brown carbon (BrC) are light‐absorbing aerosols with significant climate impacts, but their absorption properties and direct radiative effect (DRE) remain uncertain. We simulated BC and BrC absorption during the intense Canadian boreal wildfires in June 2023 using an enhanced version of CHIMERE chemical and transport model. The study focused on a domain extending from North America to Eastern Europe, including the Arctic up to 85°N. The enhanced model includes an update treatment for BC absorption enhancement and a BrC aging scheme accounting for browning and blanching through oxidation. Validation against Aerosol Robotic Network and satellite data showed the model accurately reproduced aerosol optical depth (AOD) at multiple wavelengths, both near wildfire sources and during transoceanic transport to Europe. Improvements were observed in simulations of absorbing aerosol optical depth (AAOD) compared with the baseline model. Significant enhancements were achieved in capturing the spatial distribution of aerosol absorption in areas affected by wildfire emissions. For June 2023, the regional all‐sky DRE attributed to Canadian wildfires was reduced from −2.1 W/m 2 in the control model to −1.9 W/m 2 in the enhanced model. This corresponded to an additional warming effect of +0.2 W/m 2 (+10%) due to the advanced treatment of BC and BrC absorption. These results indicate the importance of accurate aerosol absorption modeling in regional climate predictions, during large‐scale biomass burning events. They also highlight potential overestimations of cooling effects in traditional models, emphasizing the need of improved aerosol parameterization to better simulate the DRE and for evaluating the impacts of mitigation strategies.

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Publication Details

Journal
Journal of Geophysical Research Atmospheres
Published
2025-03-29
DOI
https://doi.org/10.1029/2024jd042674
Citations
4
Primary Topic
Fire effects on ecosystems
Type
article
Field-Weighted Citation Impact
4.42
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article

Modeling the Black and Brown Carbon Absorption and Their Radiative Impact: The June 2023 Intense Canadian Boreal Wildfires Case Study

Ludovico Di Antonio, Laurent Menut, Paolo Tuccella, Valentina Colaiuda et al.
4 citations
Journal of Geophysical Research Atmospheres
Fire effects on ecosystems
4.42
article

Modeling the Black and Brown Carbon Absorption and Their Radiative Impact: The June 2023 Intense Canadian Boreal Wildfires Case Study

Ludovico Di Antonio, Laurent Menut, Paolo Tuccella, Valentina Colaiuda, Raffaele Lidori, Giovanni Pitari, Edoardo Raparelli, Andrea Di Muzio
article en
4 citations

Abstract

Abstract Black carbon (BC) and brown carbon (BrC) are light‐absorbing aerosols with significant climate impacts, but their absorption properties and direct radiative effect (DRE) remain uncertain. We simulated BC and BrC absorption during the intense Canadian boreal wildfires in June 2023 using an enhanced version of CHIMERE chemical and transport model. The study focused on a domain extending from North America to Eastern Europe, including the Arctic up to 85°N. The enhanced model includes an update treatment for BC absorption enhancement and a BrC aging scheme accounting for browning and blanching through oxidation. Validation against Aerosol Robotic Network and satellite data showed the model accurately reproduced aerosol optical depth (AOD) at multiple wavelengths, both near wildfire sources and during transoceanic transport to Europe. Improvements were observed in simulations of absorbing aerosol optical depth (AAOD) compared with the baseline model. Significant enhancements were achieved in capturing the spatial distribution of aerosol absorption in areas affected by wildfire emissions. For June 2023, the regional all‐sky DRE attributed to Canadian wildfires was reduced from −2.1 W/m 2 in the control model to −1.9 W/m 2 in the enhanced model. This corresponded to an additional warming effect of +0.2 W/m 2 (+10%) due to the advanced treatment of BC and BrC absorption. These results indicate the importance of accurate aerosol absorption modeling in regional climate predictions, during large‐scale biomass burning events. They also highlight potential overestimations of cooling effects in traditional models, emphasizing the need of improved aerosol parameterization to better simulate the DRE and for evaluating the impacts of mitigation strategies.

Journal of Geophysical Research AtmospheresVol. 130(7)
Agenzia Regionale per la Protezione Ambientale del Piemonte (IT), Centre National de la Recherche Scientifique (FR), École Polytechnique (FR), Université de Versailles Saint-Quentin-en-Yvelines (FR), Université Paris-Est Créteil (FR), Université Paris Cité (FR), University of L'Aquila (IT), Université Paris Sciences et Lettres (FR), Paris-Est Sup (FR), École Normale Supérieure - PSL (FR), Sorbonne Université (FR), Institut Pierre-Simon Laplace (FR), Laboratoire Interuniversitaire des Systèmes Atmosphériques (FR), Laboratoire atmosphères, milieux, observations spatiales (FR), Laboratoire Techniques, Territoires et Sociétés (FR)
Climate action
Openalex Percentile: Top 6%
Fire effects on ecosystems
4.42
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