Directional Light Scattering of a Single Si Nanoparticle Revealed by Three-Dimensional Near-Field Optical Microscopy

Manipulation of light propagation is indispensable for the development of photonic circuits and nano-optical devices. In this study, we investigated the optical properties of Mie resonances in a single Si nanoparticle via dark field and near-field optical microscopy. The dark field spectrum of the nanoparticle exhibits electric and magnetic dipolar modes in the visible to near-infrared spectral region. The near-field spectrum shows red-shifted and enhanced peaks due to these resonances. From the electromagnetic simulation, we revealed that these unique near-field characteristics originate from the constructive interaction of the incident and scattered fields. We also performed three-dimensional near-field microscopy and demonstrated that the magnetic dipolar mode results in wider spatial extension and directional forward scattering than does the electric dipolar mode does. These findings indicate that the interaction of the magnetic dipolar mode with near-field light is desirable for controlling light propagation in various applications.

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Publication Details

Journal
The Journal of Physical Chemistry Letters
Published
2025-03-31
DOI
https://doi.org/10.1021/acs.jpclett.5c00254
Primary Topic
Near-Field Optical Microscopy
Type
article
Field-Weighted Citation Impact
0.00

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article

Directional Light Scattering of a Single Si Nanoparticle Revealed by Three-Dimensional Near-Field Optical Microscopy

Takuya Matsuura, Kohei Imura
The Journal of Physical Chemistry Letters
Near-Field Optical Microscopy
article

Directional Light Scattering of a Single Si Nanoparticle Revealed by Three-Dimensional Near-Field Optical Microscopy

Takuya Matsuura, Kohei Imura
article en

Abstract

Manipulation of light propagation is indispensable for the development of photonic circuits and nano-optical devices. In this study, we investigated the optical properties of Mie resonances in a single Si nanoparticle via dark field and near-field optical microscopy. The dark field spectrum of the nanoparticle exhibits electric and magnetic dipolar modes in the visible to near-infrared spectral region. The near-field spectrum shows red-shifted and enhanced peaks due to these resonances. From the electromagnetic simulation, we revealed that these unique near-field characteristics originate from the constructive interaction of the incident and scattered fields. We also performed three-dimensional near-field microscopy and demonstrated that the magnetic dipolar mode results in wider spatial extension and directional forward scattering than does the electric dipolar mode does. These findings indicate that the interaction of the magnetic dipolar mode with near-field light is desirable for controlling light propagation in various applications.

The Journal of Physical Chemistry LettersVol. 16(14)
Waseda University (JP)
Japan Society for the Promotion of Science, JST-Mirai Program
Openalex Percentile: Top 94%
Near-Field Optical Microscopy
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Directional Light Scattering of a Single Si Nanoparticle Revealed by Three-Dimensional Near-Field Optical Microscopy — Takuya Matsuura, Kohei Imura · The Journal of Physical Chemistry Letters (2025) | TGRS Research Map | TGRS