Successive Antiferromagnetic Transition in the Frustrated Compound CeMgIn

We report on the magnetic, transport, and thermal properties of the hexagonal ZrNiAl-type compound CeMgIn with Ce atoms forming a distorted kagome network. This compound exhibits successive antiferromagnetic transition at $T_\text{N1} =$ 2.1 K, $T_\text{N2} =$ 1.7 K, and possibly $T_\text{N3} =$ 1.3 K. The electrical resistivity exhibits a minimum at 11 K and a nonlogarithmic increase with decreasing temperature down to $T_\text{N2}$. We found that CeMgIn is the first ZrNiAl-type compound whose resistivity increase can be well explained by considering a model in which the electron-spin scattering is enhanced by the magnetic frustration and the Ruderman-Kittel-Kasuya-Yosida interaction. These results suggest that CeMgIn is a notable compound whose physical properties are strongly affected by geometrical frustration. Since the Sommerfeld coefficient is 97 mJ/mol K$^2$, CeMgIn is classified as a moderate heavy-fermion compound.

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Journal
Journal of the Physical Society of Japan
Published
2025-03-31
DOI
https://doi.org/10.7566/jpsj.94.044706
Primary Topic
Rare-earth and actinide compounds
Type
article
Field-Weighted Citation Impact
0.00

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article

Successive Antiferromagnetic Transition in the Frustrated Compound CeMgIn

Hitoshi Sugawara, Eiichi Matsuoka, Keita Onishi, Hitoshi Ohta et al.
Journal of the Physical Society of Japan
Rare-earth and actinide compounds
article

Successive Antiferromagnetic Transition in the Frustrated Compound CeMgIn

Hitoshi Sugawara, Eiichi Matsuoka, Keita Onishi, Hitoshi Ohta, Takahiro Sakurai
article en

Abstract

We report on the magnetic, transport, and thermal properties of the hexagonal ZrNiAl-type compound CeMgIn with Ce atoms forming a distorted kagome network. This compound exhibits successive antiferromagnetic transition at $T_\text{N1} =$ 2.1 K, $T_\text{N2} =$ 1.7 K, and possibly $T_\text{N3} =$ 1.3 K. The electrical resistivity exhibits a minimum at 11 K and a nonlogarithmic increase with decreasing temperature down to $T_\text{N2}$. We found that CeMgIn is the first ZrNiAl-type compound whose resistivity increase can be well explained by considering a model in which the electron-spin scattering is enhanced by the magnetic frustration and the Ruderman-Kittel-Kasuya-Yosida interaction. These results suggest that CeMgIn is a notable compound whose physical properties are strongly affected by geometrical frustration. Since the Sommerfeld coefficient is 97 mJ/mol K$^2$, CeMgIn is classified as a moderate heavy-fermion compound.

Journal of the Physical Society of JapanVol. 94(4)
Kobe University (JP)
Japan Society for the Promotion of Science, Japan Science and Technology Agency
Zero hunger
Openalex Percentile: Top 96%
Rare-earth and actinide compounds
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Successive Antiferromagnetic Transition in the Frustrated Compound CeMgIn — Hitoshi Sugawara, Eiichi Matsuoka, et al. · Journal of the Physical Society of Japan (2025) | TGRS Research Map | TGRS