Successive Antiferromagnetic Transition in the Frustrated Compound CeMgIn
We report on the magnetic, transport, and thermal properties of the hexagonal ZrNiAl-type compound CeMgIn with Ce atoms forming a distorted kagome network. This compound exhibits successive antiferromagnetic transition at $T_\text{N1} =$ 2.1 K, $T_\text{N2} =$ 1.7 K, and possibly $T_\text{N3} =$ 1.3 K. The electrical resistivity exhibits a minimum at 11 K and a nonlogarithmic increase with decreasing temperature down to $T_\text{N2}$. We found that CeMgIn is the first ZrNiAl-type compound whose resistivity increase can be well explained by considering a model in which the electron-spin scattering is enhanced by the magnetic frustration and the Ruderman-Kittel-Kasuya-Yosida interaction. These results suggest that CeMgIn is a notable compound whose physical properties are strongly affected by geometrical frustration. Since the Sommerfeld coefficient is 97 mJ/mol K$^2$, CeMgIn is classified as a moderate heavy-fermion compound.
Authors
- Hitoshi Sugawara (ORCID: https://orcid.org/0000-0002-5060-9020)
- Eiichi Matsuoka
- Keita Onishi
- Hitoshi Ohta (ORCID: https://orcid.org/0000-0001-6740-4139)
- Takahiro Sakurai (ORCID: https://orcid.org/0000-0002-1867-4682)
Institutions
- Kobe University (JP)
Publication Details
- Journal
- Journal of the Physical Society of Japan
- Published
- 2025-03-31
- DOI
- https://doi.org/10.7566/jpsj.94.044706
- Primary Topic
- Rare-earth and actinide compounds
- Type
- article
- Field-Weighted Citation Impact
- 0.00
Funders
- Japan Society for the Promotion of Science
- Japan Science and Technology Agency