Colloidal‐quantum‐dot nanolaser oscillating at a bound‐state‐in‐the‐continuum with planar surface topography for a high <i>Q</i> ‐factor

Solution-based optical gain materials offer a cost-effective path to coherent light sources. Further, bound states in the continuum (BICs) have garnered great interest owing to their diverging quality (<i>Q</i>) factors. Therefore, a hybrid of these - a solution-based material for optical gain and a BIC structure for the lasing mode - should constitute an ideal form factor for low-cost and low-threshold nanolasers. However, the nonuniform surface topography induced during the thin-film formation of a solution-based material, especially on top of a prepatterned substrate, can easily disrupt the structural symmetry required for a high-<i>Q</i> BIC, resulting in a degradation of <i>Q</i>. Thus, in this study, a simple surface-flattening technique utilizing a soft and flexible squeegee was applied, which realized the planar surface topography crucial for preserving the high <i>Q</i> promised by the BIC and achieving low-threshold lasing. We fabricated BIC nanolasers by incorporating colloidal quantum dots (CQDs) for optical gain into a two-dimensional photonic crystal backbone layer composed of Si<sub>3</sub>N<sub>4</sub>. By leveraging the unique properties of the BIC mode with a well-ordered surface, our CQD-based BIC laser exhibited a lasing threshold as low as 10.5 kW/cm<sup>2</sup>, which is significantly lower than those reported in previous studies.

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Publication Details

Journal
Nanophotonics
Published
2025-03-29
DOI
https://doi.org/10.1515/nanoph-2024-0730
Citations
6
Primary Topic
Photonic Crystals and Applications
Type
article
Field-Weighted Citation Impact
7.48

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article

Colloidal‐quantum‐dot nanolaser oscillating at a bound‐state‐in‐the‐continuum with planar surface topography for a high Q ‐factor

Heonsu Jeon, Tae‐Yun Lee, Hansol Lee
6 citations
Nanophotonics
Photonic Crystals and Applications
7.48
article

Colloidal‐quantum‐dot nanolaser oscillating at a bound‐state‐in‐the‐continuum with planar surface topography for a high Q ‐factor

Heonsu Jeon, Tae‐Yun Lee, Hansol Lee
article en
6 citations

Abstract

Solution-based optical gain materials offer a cost-effective path to coherent light sources. Further, bound states in the continuum (BICs) have garnered great interest owing to their diverging quality (<i>Q</i>) factors. Therefore, a hybrid of these - a solution-based material for optical gain and a BIC structure for the lasing mode - should constitute an ideal form factor for low-cost and low-threshold nanolasers. However, the nonuniform surface topography induced during the thin-film formation of a solution-based material, especially on top of a prepatterned substrate, can easily disrupt the structural symmetry required for a high-<i>Q</i> BIC, resulting in a degradation of <i>Q</i>. Thus, in this study, a simple surface-flattening technique utilizing a soft and flexible squeegee was applied, which realized the planar surface topography crucial for preserving the high <i>Q</i> promised by the BIC and achieving low-threshold lasing. We fabricated BIC nanolasers by incorporating colloidal quantum dots (CQDs) for optical gain into a two-dimensional photonic crystal backbone layer composed of Si<sub>3</sub>N<sub>4</sub>. By leveraging the unique properties of the BIC mode with a well-ordered surface, our CQD-based BIC laser exhibited a lasing threshold as low as 10.5 kW/cm<sup>2</sup>, which is significantly lower than those reported in previous studies.

NanophotonicsVol. 14(10)
Seoul National University (KR), Seoul Semiconductor (South Korea) (KR)
National Research Foundation of Korea, Samsung
Openalex Percentile: Top 3%
Photonic Crystals and Applications
7.48
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