Strong Damping-Like Torques in Wafer-Scale MoTe<sub><b>2</b></sub> Grown by MOCVD
The scalable synthesis of materials with strong spin orbit coupling (SOC) is crucial for the development of spintronic and magnetic devices. Here, wafer-scale growth of 1T' MoTe<sub>2</sub> using metal-organic chemical vapor deposition (MOCVD) at low temperatures (400 °C) is demonstrated. The synthesized films exhibit uniform coverage across the entire substrate, as well as accurate stoichiometry. This low-temperature synthesis is compatible with silicon back-end-of-line (BEOL) processes, enabling in-memory and in-sensor computing for data-intensive applications. Furthermore, it was found that the grown 1T' MoTe<sub>2</sub> exhibits strong spin-orbit coupling, as revealed by the spin torque ferromagnetic resonance (ST-FMR) measurements conducted on a 1T' MoTe<sub>2</sub>/permalloy bilayer. These measurements indicate significant damping-like torques in the wafer-scale 1T' MoTe<sub>2</sub> film and indicate high spin-charge conversion efficiency. The BEOL-compatible process and potent spin orbit torque demonstrate the promise of MOCVD-grown MoTe<sub>2</sub> in advanced device applications.
Authors
- A. Hoffmann (ORCID: https://orcid.org/0000-0002-6800-4169)
- Marwan Eladl
- Wenjuan Zhu (ORCID: https://orcid.org/0000-0003-2824-1386)
- Hanwool Lee (ORCID: https://orcid.org/0000-0002-8990-6022)
- Stasiu T. Chyczewski (ORCID: https://orcid.org/0000-0003-3461-998X)
- Shuchen Li (ORCID: https://orcid.org/0000-0003-1626-9533)
- Jun‐Fei Zheng
Institutions
- University of Illinois Urbana-Champaign (US)
- Entegris (United States) (US)
- Division of Materials Science and Engineering (AU)
Publication Details
- Journal
- ACS Applied Materials & Interfaces
- Published
- 2025-03-28
- DOI
- https://doi.org/10.1021/acsami.4c21247
- Citations
- 2
- Primary Topic
- 2D Materials and Applications
- Type
- article
- Field-Weighted Citation Impact
- 1.04
Funders
- Air Force Office of Scientific Research