Temporal interference picture for subpeak structures between Autler-Townes doublets in photoelectron energy spectra

The existence of subpeak structures between the Autler-Townes (AT) doublet of the photoelectron spectrum during resonant ionization of an atom has been predicted in a large number of theoretical calculations, but a convincing physical explanation is still lacking. In this study we establish a temporal interference picture to elucidate the physical origin of these subpeaks. We derive an analytical estimation for the photoelectron spectra based on a three-level model, which agrees well with the numerical solution of the time-dependent Schr"odinger equation at moderately strong pulse intensities. Our interpretation suggests that the interference of the photoelectron wave packet emitted during each Rabi cycle results in the subpeak structure between the AT doublet. By analyzing the phase difference between two temporally adjacent photoelectron wave packets, we successfully predict the interference minima in the photoelectron energy spectra.

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Publication Details

Journal
Physical review. A/Physical review, A
Published
2025-03-28
DOI
https://doi.org/10.1103/physreva.111.033117
Citations
4
Primary Topic
Electron and X-Ray Spectroscopy Techniques
Type
article
Field-Weighted Citation Impact
2.64

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article

Temporal interference picture for subpeak structures between Autler-Townes doublets in photoelectron energy spectra

Guangyin Liu, Weijun Wan, Wei‐Chao Jiang, Meng-Fei Xie et al.
4 citations
Physical review. A/Physical review, A
Electron and X-Ray Spectroscopy Techniques
2.64
article

Temporal interference picture for subpeak structures between Autler-Townes doublets in photoelectron energy spectra

Guangyin Liu, Weijun Wan, Wei‐Chao Jiang, Meng-Fei Xie, Q. Meng
article en
4 citations

Abstract

The existence of subpeak structures between the Autler-Townes (AT) doublet of the photoelectron spectrum during resonant ionization of an atom has been predicted in a large number of theoretical calculations, but a convincing physical explanation is still lacking. In this study we establish a temporal interference picture to elucidate the physical origin of these subpeaks. We derive an analytical estimation for the photoelectron spectra based on a three-level model, which agrees well with the numerical solution of the time-dependent Schr\"odinger equation at moderately strong pulse intensities. Our interpretation suggests that the interference of the photoelectron wave packet emitted during each Rabi cycle results in the subpeak structure between the AT doublet. By analyzing the phase difference between two temporally adjacent photoelectron wave packets, we successfully predict the interference minima in the photoelectron energy spectra.

Physical review. A/Physical review, AVol. 111(3)
Shenzhen University (CN)
National Natural Science Foundation of China, National Key Research and Development Program of China
Affordable and clean energy
Openalex Percentile: Top 11%
Electron and X-Ray Spectroscopy Techniques
2.64
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