Plateaus in the Potentials of Density-Functional Theory: Analytical Derivation and Useful Approximations

Density functional theory (DFT) is an extremely efficient and widely used method for electronic structure calculations. However, the quality of such calculations crucially depends on the quality of the approximation used for the exchange-correlation functional, for which there is no exact form. One important feature of the exact exchange-correlation potential, which common approximations usually do not capture, is the spatial steps and plateaus that occur in various scenarios, including ionization, excitation, dissociation, and charge transfer. In this paper, we derive an analytical expression for the plateau in the Kohn-Sham potential that forms around the center of the system, when the number of electrons infinitesimally surpasses an integer. The resulting formula is the first analytical expression of its kind. The derivation is performed using the orbital-free DFT framework, analyzing both the Kohn-Sham-Pauli and the Pauli potentials. Analytical results are compared to exact calculations for small atomic systems, showing close correspondence and high accuracy. Furthermore, it is shown that plateaus can be produced also when relying on approximate electron densities, even those obtained with the simplest exchange-correlation form─the local density approximation.

Authors

Institutions

Publication Details

Journal
Journal of Chemical Theory and Computation
Published
2025-03-27
DOI
https://doi.org/10.1021/acs.jctc.4c01771
Citations
2
Primary Topic
Advanced Thermodynamics and Statistical Mechanics
Type
article
Field-Weighted Citation Impact
2.65
Controls
|||
ALL TIME
JAN
FEB
MAR
APR
MAY
JUN
JUL
AUG
SEP
OCT
article

Plateaus in the Potentials of Density-Functional Theory: Analytical Derivation and Useful Approximations

Eli Kraisler, Nathan E. Rahat
2 citations
Journal of Chemical Theory and Computation
Advanced Thermodynamics and Statistical Mechanics
2.65
article

Plateaus in the Potentials of Density-Functional Theory: Analytical Derivation and Useful Approximations

Eli Kraisler, Nathan E. Rahat
article en
2 citations

Abstract

Density functional theory (DFT) is an extremely efficient and widely used method for electronic structure calculations. However, the quality of such calculations crucially depends on the quality of the approximation used for the exchange-correlation functional, for which there is no exact form. One important feature of the exact exchange-correlation potential, which common approximations usually do not capture, is the spatial steps and plateaus that occur in various scenarios, including ionization, excitation, dissociation, and charge transfer. In this paper, we derive an analytical expression for the plateau in the Kohn-Sham potential that forms around the center of the system, when the number of electrons infinitesimally surpasses an integer. The resulting formula is the first analytical expression of its kind. The derivation is performed using the orbital-free DFT framework, analyzing both the Kohn-Sham-Pauli and the Pauli potentials. Analytical results are compared to exact calculations for small atomic systems, showing close correspondence and high accuracy. Furthermore, it is shown that plateaus can be produced also when relying on approximate electron densities, even those obtained with the simplest exchange-correlation form─the local density approximation.

Journal of Chemical Theory and ComputationVol. 21(7)
Hebrew University of Jerusalem (IL)
Openalex Percentile: Top 12%
Advanced Thermodynamics and Statistical Mechanics
2.65
AI Navigator

Ask Laika to Summarize, Analyze, and Connect papers live on the map.

Summarize Papers & Methodologies

Extract key findings, datasets, and comparative methods across publications.

Benchmark Rankings & Visual Analytics

Rank top research institutions, authors, funders, topics, and journals by Field-Weighted Citation Impact (FWCI) and paper volume with instant charts.

Connect Distant Disciplines

Bridge topological clusters on the map to find hidden collaborative intersections.

Plateaus in the Potentials of Density-Functional Theory: Analytical Derivation and Useful Approximations — Eli Kraisler, Nathan E. Rahat · Journal of Chemical Theory and Computation (2025) | TGRS Research Map | TGRS