Magnetization process of a quasi-two-dimensional quantum magnet: Two-step symmetry restoration and dimensional reduction

We report on a comprehensive thermodynamic study of a quasi-two-dimensional (quasi-2D) quantum magnet ${\mathrm{Cu}}_{2}{(\mathrm{OH})}_{3}\mathrm{Br}$ which in the 2D layer can be viewed as strongly coupled alternating antiferromagnetic and ferromagnetic chains. In an applied magnetic field transverse to the ordered spins below ${T}_{N}=9.3$ K, a field-induced phase transition from the 3D ordered to a disordered phase occurs at ${B}_{c}=16.3$ T for the lowest temperature, which is featured by an onset of a one-half plateaulike magnetization. By performing quantum Monte Carlo simulations of the relevant 2D model, we find that the plateaulike magnetization corresponds to a partial symmetry restoration and the full polarization in the ferromagnetic chains. Our numerical simulations also show that the magnetization saturation occurs with full symmetry restoration at a much higher field of ${B}_{s}\ensuremath{\simeq}95$ T, corresponding to a 1D quantum phase transition in the antiferromagnetic chains. We argue that the experimentally observed field-induced phase transition at ${B}_{c}$ follows from the partial symmetry restoration and the concomitant dimensional reduction.