Wavelength-resolved neutron transmission analyses of textured materials

Wavelength-resolved neutron imaging for diffraction contrast often referred to as Bragg edge imaging is a neutron-based technique that has gained attention in recent years due to its promising ability to characterize the microstructure of polycrystalline materials with spatial resolution. This method relies on spatially resolved analyses of diffraction induced features in transmission spectra within the thermal neutron range. Assessable characteristics are e.g. phase fractions, lattice strains, and crystallographic texture. For the latter forward modelling of transmission spectra from known orientation distribution functions (ODFs) has been demonstrated for various materials. However, solving the inverse problem—retrieving crystallographic texture from transmission spectra—presents a more complex challenge. In recent years, the authors have developed two theoretical approaches to model the relationship between transmission spectra and texture, either by decomposing the ODF into individual orientation fractions or by expanding it into a Fourier series. Both approaches have shown excellent predictive capability for materials with different crystal symmetries, including hexagonal, FCC, and BCC structures. Here we present the comparison between the proposed models, highlighting the advantages and disadvantages of the direct method based on different approaches for the analysis of wavelength-resolved neutron transmission experiments of textured materials. Finally, we present the future trends in the inversion method, i.e., the estimation of the ODFs from transmission spectra in tomography experiments. • Wavelength-resolved neutron imaging models for textured specimens. • Neutron transmission simulation of textured materials from known ODFs and comparison with experimental data. • Discussion of ODFs estimation from transmission spectra in tomography experiments.

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Publication Details

Journal
Materials Characterization
Published
2025-03-24
DOI
https://doi.org/10.1016/j.matchar.2025.114969
Citations
2
Primary Topic
Nuclear Physics and Applications
Type
article
Field-Weighted Citation Impact
3.77
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article

Wavelength-resolved neutron transmission analyses of textured materials

J.R. Santisteban, Florencia Malamud, Markus Ströbl, M.A. Vicente Álvarez
2 citations
Materials Characterization
Nuclear Physics and Applications
3.77
article

Wavelength-resolved neutron transmission analyses of textured materials

J.R. Santisteban, Florencia Malamud, Markus Ströbl, M.A. Vicente Álvarez
article en
2 citations

Abstract

Wavelength-resolved neutron imaging for diffraction contrast often referred to as Bragg edge imaging is a neutron-based technique that has gained attention in recent years due to its promising ability to characterize the microstructure of polycrystalline materials with spatial resolution. This method relies on spatially resolved analyses of diffraction induced features in transmission spectra within the thermal neutron range. Assessable characteristics are e.g. phase fractions, lattice strains, and crystallographic texture. For the latter forward modelling of transmission spectra from known orientation distribution functions (ODFs) has been demonstrated for various materials. However, solving the inverse problem—retrieving crystallographic texture from transmission spectra—presents a more complex challenge. In recent years, the authors have developed two theoretical approaches to model the relationship between transmission spectra and texture, either by decomposing the ODF into individual orientation fractions or by expanding it into a Fourier series. Both approaches have shown excellent predictive capability for materials with different crystal symmetries, including hexagonal, FCC, and BCC structures. Here we present the comparison between the proposed models, highlighting the advantages and disadvantages of the direct method based on different approaches for the analysis of wavelength-resolved neutron transmission experiments of textured materials. Finally, we present the future trends in the inversion method, i.e., the estimation of the ODFs from transmission spectra in tomography experiments. • Wavelength-resolved neutron imaging models for textured specimens. • Neutron transmission simulation of textured materials from known ODFs and comparison with experimental data. • Discussion of ODFs estimation from transmission spectra in tomography experiments.

Materials CharacterizationVol. 223
Paul Scherrer Institute (CH), Bariloche Atomic Centre (AR), Centro Científico Tecnológico - San Juan (AR)
Climate action
Openalex Percentile: Top 9%
Nuclear Physics and Applications
3.77
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