Bandwidth of Lightwave-Driven Electronic Response from Metallic Nanoantennas

Lightwave electronics offer transformative field-level precision and control at high optical frequencies. While recent advances show that lightwave-driven electron emission from nanoantennas enables time-domain, field-resolved analysis of optical waveforms through a small-signal analysis, the effect of the gate waveform on the measurement transfer function remains unexplored. By generating electrons with a 10-cycle pulse in the optical tunneling regime and perturbing the response with a 1.5-cycle pulse, we experimentally measure the bandwidth limitations imposed by the electron emission process. By comparing these measurements with TDSE simulations and analytical models, we reveal the temporal properties of the electronic response and its impact on the small-signal transfer function. Our results test and confirm the accuracy of the Fowler-Nordheim model in estimating the lightwave electronic response from noble metals. We envision extending these techniques to multi-octave-spanning signals for precise characterization of sub-cycle electronic responses through harmonic frequency mixing.

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Publication Details

Journal
Nano Letters
Published
2025-03-24
DOI
https://doi.org/10.1021/acs.nanolett.4c06536
Citations
2
Primary Topic
Plasmonic and Surface Plasmon Research
Type
article
Field-Weighted Citation Impact
1.35

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article

Bandwidth of Lightwave-Driven Electronic Response from Metallic Nanoantennas

Karl K. Berggren, Marco Turchetti, Felix Ritzkowsky, Shih‐Hsuan Chia et al.
2 citations
Nano Letters
Plasmonic and Surface Plasmon Research
1.35
article

Bandwidth of Lightwave-Driven Electronic Response from Metallic Nanoantennas

Karl K. Berggren, Marco Turchetti, Felix Ritzkowsky, Shih‐Hsuan Chia, Matthew Yeung, Lu‐Ting Chou, Phillip D. Keathley
article en
2 citations

Abstract

Lightwave electronics offer transformative field-level precision and control at high optical frequencies. While recent advances show that lightwave-driven electron emission from nanoantennas enables time-domain, field-resolved analysis of optical waveforms through a small-signal analysis, the effect of the gate waveform on the measurement transfer function remains unexplored. By generating electrons with a 10-cycle pulse in the optical tunneling regime and perturbing the response with a 1.5-cycle pulse, we experimentally measure the bandwidth limitations imposed by the electron emission process. By comparing these measurements with TDSE simulations and analytical models, we reveal the temporal properties of the electronic response and its impact on the small-signal transfer function. Our results test and confirm the accuracy of the Fowler-Nordheim model in estimating the lightwave electronic response from noble metals. We envision extending these techniques to multi-octave-spanning signals for precise characterization of sub-cycle electronic responses through harmonic frequency mixing.

Nano LettersVol. 25(13)
National Yang Ming Chiao Tung University (TW), Massachusetts Institute of Technology (US)
Alexander von Humboldt-Stiftung, National Science and Technology Council, Directorate for Mathematical and Physical Sciences
Affordable and clean energy
Openalex Percentile: Top 21%
Plasmonic and Surface Plasmon Research
1.35
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Bandwidth of Lightwave-Driven Electronic Response from Metallic Nanoantennas — Karl K. Berggren, Marco Turchetti, et al. · Nano Letters (2025) | TGRS Research Map | TGRS